Li, X., Wu, G., Zhang, L., Huang, D., Li, Y., Zhang, R., Li, M., Zhu, L., Guo, J., Huang, T., Shen, J., Wei, X., Yu, K. M., Dong, J., Altman, M. S., Ruoff, R. S., Duan, Y., Yu, J., Wang, Z., ... Tang, W. (2022). Single-crystal two-dimensional material epitaxy on tailored non-single-crystal substrates. Nature Communications, 13(1), 文章 1773. https://doi.org/10.1038/s41467-022-29451-w
Li, Xin ; Wu, Guilin ; Zhang, Leining 等. / Single-crystal two-dimensional material epitaxy on tailored non-single-crystal substrates. 在: Nature Communications. 2022 ; 卷 13, 号码 1.
@article{5700d7aece584b3f8c750d6f97de58bd,
title = "Single-crystal two-dimensional material epitaxy on tailored non-single-crystal substrates",
abstract = "The use of single-crystal substrates as templates for the epitaxial growth of single-crystal overlayers has been a primary principle of materials epitaxy for more than 70 years. Here we report our finding that, though counterintuitive, single-crystal 2D materials can be epitaxially grown on twinned crystals. By establishing a geometric principle to describe 2D materials alignment on high-index surfaces, we show that 2D material islands grown on the two sides of a twin boundary can be well aligned. To validate this prediction, wafer-scale Cu foils with abundant twin boundaries were synthesized, and on the surfaces of these polycrystalline Cu foils, we have successfully grown wafer-scale single-crystal graphene and hexagonal boron nitride films. In addition, to greatly increasing the availability of large area high-quality 2D single crystals, our discovery also extends the fundamental understanding of materials epitaxy.",
author = "Xin Li and Guilin Wu and Leining Zhang and Deping Huang and Yunqing Li and Ruiqi Zhang and Meng Li and Lin Zhu and Jing Guo and Tianlin Huang and Jun Shen and Xingzhan Wei and Yu, {Ka Man} and Jichen Dong and Altman, {Michael S.} and Ruoff, {Rodney S.} and Yinwu Duan and Jie Yu and Zhujun Wang and Xiaoxu Huang and Feng Ding and Haofei Shi and Wenxin Tang",
note = "Publisher Copyright: {\textcopyright} 2022, The Author(s).",
year = "2022",
month = dec,
doi = "10.1038/s41467-022-29451-w",
language = "English",
volume = "13",
journal = "Nature Communications",
issn = "2041-1723",
publisher = "Nature Publishing Group",
number = "1",
}
Li, X, Wu, G, Zhang, L, Huang, D, Li, Y, Zhang, R, Li, M, Zhu, L, Guo, J, Huang, T, Shen, J, Wei, X, Yu, KM, Dong, J, Altman, MS, Ruoff, RS, Duan, Y, Yu, J, Wang, Z, Huang, X, Ding, F, Shi, H & Tang, W 2022, 'Single-crystal two-dimensional material epitaxy on tailored non-single-crystal substrates', Nature Communications, 卷 13, 号码 1, 1773. https://doi.org/10.1038/s41467-022-29451-w
Single-crystal two-dimensional material epitaxy on tailored non-single-crystal substrates. / Li, Xin; Wu, Guilin
; Zhang, Leining 等.
在:
Nature Communications, 卷 13, 号码 1, 1773, 12.2022.
科研成果: 期刊稿件 › 文章 › 同行评审
TY - JOUR
T1 - Single-crystal two-dimensional material epitaxy on tailored non-single-crystal substrates
AU - Li, Xin
AU - Wu, Guilin
AU - Zhang, Leining
AU - Huang, Deping
AU - Li, Yunqing
AU - Zhang, Ruiqi
AU - Li, Meng
AU - Zhu, Lin
AU - Guo, Jing
AU - Huang, Tianlin
AU - Shen, Jun
AU - Wei, Xingzhan
AU - Yu, Ka Man
AU - Dong, Jichen
AU - Altman, Michael S.
AU - Ruoff, Rodney S.
AU - Duan, Yinwu
AU - Yu, Jie
AU - Wang, Zhujun
AU - Huang, Xiaoxu
AU - Ding, Feng
AU - Shi, Haofei
AU - Tang, Wenxin
N1 - Publisher Copyright:
© 2022, The Author(s).
PY - 2022/12
Y1 - 2022/12
N2 - The use of single-crystal substrates as templates for the epitaxial growth of single-crystal overlayers has been a primary principle of materials epitaxy for more than 70 years. Here we report our finding that, though counterintuitive, single-crystal 2D materials can be epitaxially grown on twinned crystals. By establishing a geometric principle to describe 2D materials alignment on high-index surfaces, we show that 2D material islands grown on the two sides of a twin boundary can be well aligned. To validate this prediction, wafer-scale Cu foils with abundant twin boundaries were synthesized, and on the surfaces of these polycrystalline Cu foils, we have successfully grown wafer-scale single-crystal graphene and hexagonal boron nitride films. In addition, to greatly increasing the availability of large area high-quality 2D single crystals, our discovery also extends the fundamental understanding of materials epitaxy.
AB - The use of single-crystal substrates as templates for the epitaxial growth of single-crystal overlayers has been a primary principle of materials epitaxy for more than 70 years. Here we report our finding that, though counterintuitive, single-crystal 2D materials can be epitaxially grown on twinned crystals. By establishing a geometric principle to describe 2D materials alignment on high-index surfaces, we show that 2D material islands grown on the two sides of a twin boundary can be well aligned. To validate this prediction, wafer-scale Cu foils with abundant twin boundaries were synthesized, and on the surfaces of these polycrystalline Cu foils, we have successfully grown wafer-scale single-crystal graphene and hexagonal boron nitride films. In addition, to greatly increasing the availability of large area high-quality 2D single crystals, our discovery also extends the fundamental understanding of materials epitaxy.
UR - http://www.scopus.com/inward/record.url?scp=85127373219&partnerID=8YFLogxK
U2 - 10.1038/s41467-022-29451-w
DO - 10.1038/s41467-022-29451-w
M3 - Article
C2 - 35365650
AN - SCOPUS:85127373219
SN - 2041-1723
VL - 13
JO - Nature Communications
JF - Nature Communications
IS - 1
M1 - 1773
ER -
Li X, Wu G, Zhang L, Huang D, Li Y, Zhang R 等. Single-crystal two-dimensional material epitaxy on tailored non-single-crystal substrates. Nature Communications. 2022 12月;13(1):1773. doi: 10.1038/s41467-022-29451-w