Quantitative determination of hydrogen isotope in titanium using LIBS

Yang Du, Qianqian Wang, Ruizhu Yang, Xutai Cui

科研成果: 书/报告/会议事项章节会议稿件同行评审

4 引用 (Scopus)

摘要

In this paper, we investigated how to use calibration-free (CF) LIBS to quantitatively analyze hydrogen and deuterium in titanium samples in ambient helium gas. First, the LIBS spectra of two metal titanium samples with hydrogen (H)/deuterium (D) concentration ratios of 1.5 (0.6: 0.4) and 0.67 (0.4: 0.6) were obtained by a LIBS experiment set-up. Then, based on the Boltzmann plot of the Ti elements, the plasma electron temperatures of the two samples were determined to be 5746K and 5736K, respectively. The corresponding electron density measured by the Stark broadening profile of Ti II (375.9nm) is 7 × 1015 cm-3 and 7.73 × 1015 cm-3. According to the experimental data, the McWhirter criterion was verified and LIBS plasma was in LTE, so CF-LIBS method can be used to analyze the concentration of hydrogen isotopes. The H/D concentration ratios of the two samples were calculated using free calibration method to be 1.48 and 0.81, and the relative errors were 1.33% and 20.9%, respectively. The experimental results demostrated that laser-induced breakdown spectroscopy combined with the free calibration method can be applied in the quantitative analysis of hydrogen isotope.

源语言英语
主期刊名Applications of Digital Image Processing XLII
编辑Andrew G. Tescher, Touradj Ebrahimi
出版商SPIE
ISBN(电子版)9781510629677
DOI
出版状态已出版 - 2019
活动Applications of Digital Image Processing XLII 2019 - San Diego, 美国
期限: 12 8月 201915 8月 2019

出版系列

姓名Proceedings of SPIE - The International Society for Optical Engineering
11337
ISSN(印刷版)0277-786X
ISSN(电子版)1996-756X

会议

会议Applications of Digital Image Processing XLII 2019
国家/地区美国
San Diego
时期12/08/1915/08/19

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