Post-cyclization of a bisimine-linked covalent organic framework to enhance the performance of visible-light photocatalytic hydrogen evolution

Huanyu Liu; Yueting Li; Lu Dai; Xiangjian Meng; Anwang Dong; Zimo Zhou; Huixia Lv; Pengfei Li; Bo Wang

doi:10.1039/d3py00181d

Post-cyclization of a bisimine-linked covalent organic framework to enhance the performance of visible-light photocatalytic hydrogen evolution

Huanyu Liu, Yueting Li, Lu Dai, Xiangjian Meng, Anwang Dong, Zimo Zhou, Huixia Lv, Pengfei Li^*, Bo Wang

^*此作品的通讯作者

Beijing Institute of Technology

科研成果: 期刊稿件 › 文章 › 同行评审

3 引用（Scopus）

摘要

Covalent organic frameworks (COFs) are promising candidates for the photocatalytic hydrogen evolution. Here, we reported the synthesis of a bisimine-linked COF and its partial post-cyclization to an imidazolium-linked COF. Both the chemical stability and π-electron delocalization are significantly improved by the post-cyclization, leading to a triply increased hydrogen evolution rate.

源语言	英语
页（从-至）	1323-1329
页数	7
期刊	Polymer Chemistry
卷	14
期	12
DOI	https://doi.org/10.1039/d3py00181d
出版状态	已出版 - 9 3月 2023

访问文件

10.1039/d3py00181d

其它文件与链接

链接到 Scopus 的出版物

引用此

Liu, H., Li, Y., Dai, L., Meng, X., Dong, A., Zhou, Z., Lv, H., Li, P., & Wang, B. (2023). Post-cyclization of a bisimine-linked covalent organic framework to enhance the performance of visible-light photocatalytic hydrogen evolution. Polymer Chemistry, 14(12), 1323-1329. https://doi.org/10.1039/d3py00181d

@article{c4cd0401811f40299ea050749e1971f0,

title = "Post-cyclization of a bisimine-linked covalent organic framework to enhance the performance of visible-light photocatalytic hydrogen evolution",

abstract = "Covalent organic frameworks (COFs) are promising candidates for the photocatalytic hydrogen evolution. Here, we reported the synthesis of a bisimine-linked COF and its partial post-cyclization to an imidazolium-linked COF. Both the chemical stability and π-electron delocalization are significantly improved by the post-cyclization, leading to a triply increased hydrogen evolution rate.",

author = "Huanyu Liu and Yueting Li and Lu Dai and Xiangjian Meng and Anwang Dong and Zimo Zhou and Huixia Lv and Pengfei Li and Bo Wang",

note = "Publisher Copyright: {\textcopyright} 2023 The Royal Society of Chemistry.",

year = "2023",

month = mar,

day = "9",

doi = "10.1039/d3py00181d",

language = "English",

volume = "14",

pages = "1323--1329",

journal = "Polymer Chemistry",

issn = "1759-9954",

publisher = "Royal Society of Chemistry",

number = "12",

}

TY - JOUR

T1 - Post-cyclization of a bisimine-linked covalent organic framework to enhance the performance of visible-light photocatalytic hydrogen evolution

AU - Liu, Huanyu

AU - Li, Yueting

AU - Dai, Lu

AU - Meng, Xiangjian

AU - Dong, Anwang

AU - Zhou, Zimo

AU - Lv, Huixia

AU - Li, Pengfei

AU - Wang, Bo

PY - 2023/3/9

Y1 - 2023/3/9

N2 - Covalent organic frameworks (COFs) are promising candidates for the photocatalytic hydrogen evolution. Here, we reported the synthesis of a bisimine-linked COF and its partial post-cyclization to an imidazolium-linked COF. Both the chemical stability and π-electron delocalization are significantly improved by the post-cyclization, leading to a triply increased hydrogen evolution rate.

AB - Covalent organic frameworks (COFs) are promising candidates for the photocatalytic hydrogen evolution. Here, we reported the synthesis of a bisimine-linked COF and its partial post-cyclization to an imidazolium-linked COF. Both the chemical stability and π-electron delocalization are significantly improved by the post-cyclization, leading to a triply increased hydrogen evolution rate.

UR - http://www.scopus.com/inward/record.url?scp=85151035552&partnerID=8YFLogxK

U2 - 10.1039/d3py00181d

DO - 10.1039/d3py00181d

M3 - Article

AN - SCOPUS:85151035552

SN - 1759-9954

VL - 14

SP - 1323

EP - 1329

JO - Polymer Chemistry

JF - Polymer Chemistry

IS - 12

ER -

Post-cyclization of a bisimine-linked covalent organic framework to enhance the performance of visible-light photocatalytic hydrogen evolution

摘要

访问文件

其它文件与链接

指纹

引用此