Bilayer of polyelectrolyte films for spontaneous power generation in air up to an integrated 1,000 V output

Haiyan Wang, Yilin Sun, Tiancheng He, Yaxin Huang, Huhu Cheng*, Chun Li, Dan Xie, Pengfei Yang, Yanfeng Zhang, Liangti Qu*

*Corresponding author for this work

Research output: Contribution to journalArticlepeer-review

257 Citations (Scopus)

Abstract

Environmentally adaptive power generation is attractive for the development of next-generation energy sources. Here we develop a heterogeneous moisture-enabled electric generator (HMEG) based on a bilayer of polyelectrolyte films. Through the spontaneous adsorption of water molecules in air and induced diffusion of oppositely charged ions, one single HMEG unit can produce a high voltage of ~0.95 V at low (25%) relative humidity (RH), and even jump to 1.38 V at 85% RH. A sequentially aligned stacking strategy is created for large-scale integration of HMEG units, to offer a voltage of more than 1,000 V under ambient conditions (25% RH, 25 °C). Using origami assembly, a small section of folded HMEGs renders an output of up to 43 V cm−3. Such integration devices supply sufficient power to illuminate a lamp bulb of 10 W, to drive a dynamic electronic ink screen and to control the gate voltage for a self-powered field effect transistor.

Original languageEnglish
Pages (from-to)811-819
Number of pages9
JournalNature Nanotechnology
Volume16
Issue number7
DOIs
Publication statusPublished - Jul 2021
Externally publishedYes

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