Unusual Assembly and Conversion of Graphene Quantum Dots into Crystalline Graphite Nanocapsules

Jian Gao; Chenyu Xu; Yue Hu; Fei Zhao; Changxiang Shao; Yang Zhao; Shilv Chen; Liangti Qu

doi:10.1002/asia.201700297

Unusual Assembly and Conversion of Graphene Quantum Dots into Crystalline Graphite Nanocapsules

Jian Gao, Chenyu Xu, Yue Hu, Fei Zhao, Changxiang Shao, Yang Zhao^*, Shilv Chen, Liangti Qu

^*此作品的通讯作者

化学与化工学院

科研成果: 期刊稿件 › 文章 › 同行评审

4 引用（Scopus）

摘要

The development of a facile strategy for conversion of graphene quantum dots (GQDs) into crystalline graphite is of great practical significance and still remains challenging. Herein, rationally assembled crystalline-intercrossed graphite nanocapsules (CI-GNCs) have been realized by a one-step electrochemically induced strategy with the assistance of a soft template, in which the GQDs act as the initial building blocks. The as-prepared CI-GNCs exhibit highly crystalline graphitic nanostructures. Moreover, they possess promising electrocatalytic activity for the oxygen reaction reduction (ORR) in alkaline medium. This simple fabrication technology presents a great advance for synthesizing CI-GNCs composite catalysts, which have potential as new metal-free catalysts for efficient ORR applications.

源语言	英语
页（从-至）	1272-1276
页数	5
期刊	Chemistry - An Asian Journal
卷	12
期	12
DOI	https://doi.org/10.1002/asia.201700297
出版状态	已出版 - 19 6月 2017

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Gao, J., Xu, C., Hu, Y., Zhao, F., Shao, C., Zhao, Y., Chen, S., & Qu, L. (2017). Unusual Assembly and Conversion of Graphene Quantum Dots into Crystalline Graphite Nanocapsules. Chemistry - An Asian Journal, 12(12), 1272-1276. https://doi.org/10.1002/asia.201700297

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title = "Unusual Assembly and Conversion of Graphene Quantum Dots into Crystalline Graphite Nanocapsules",

abstract = "The development of a facile strategy for conversion of graphene quantum dots (GQDs) into crystalline graphite is of great practical significance and still remains challenging. Herein, rationally assembled crystalline-intercrossed graphite nanocapsules (CI-GNCs) have been realized by a one-step electrochemically induced strategy with the assistance of a soft template, in which the GQDs act as the initial building blocks. The as-prepared CI-GNCs exhibit highly crystalline graphitic nanostructures. Moreover, they possess promising electrocatalytic activity for the oxygen reaction reduction (ORR) in alkaline medium. This simple fabrication technology presents a great advance for synthesizing CI-GNCs composite catalysts, which have potential as new metal-free catalysts for efficient ORR applications.",

keywords = "carbon, electrocatalysis, graphene quantum dots, graphite nanocapsules, oxygen reduction reaction",

author = "Jian Gao and Chenyu Xu and Yue Hu and Fei Zhao and Changxiang Shao and Yang Zhao and Shilv Chen and Liangti Qu",

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AU - Gao, Jian

AU - Xu, Chenyu

AU - Hu, Yue

AU - Zhao, Fei

AU - Shao, Changxiang

AU - Zhao, Yang

AU - Chen, Shilv

AU - Qu, Liangti

PY - 2017/6/19

Y1 - 2017/6/19

N2 - The development of a facile strategy for conversion of graphene quantum dots (GQDs) into crystalline graphite is of great practical significance and still remains challenging. Herein, rationally assembled crystalline-intercrossed graphite nanocapsules (CI-GNCs) have been realized by a one-step electrochemically induced strategy with the assistance of a soft template, in which the GQDs act as the initial building blocks. The as-prepared CI-GNCs exhibit highly crystalline graphitic nanostructures. Moreover, they possess promising electrocatalytic activity for the oxygen reaction reduction (ORR) in alkaline medium. This simple fabrication technology presents a great advance for synthesizing CI-GNCs composite catalysts, which have potential as new metal-free catalysts for efficient ORR applications.

AB - The development of a facile strategy for conversion of graphene quantum dots (GQDs) into crystalline graphite is of great practical significance and still remains challenging. Herein, rationally assembled crystalline-intercrossed graphite nanocapsules (CI-GNCs) have been realized by a one-step electrochemically induced strategy with the assistance of a soft template, in which the GQDs act as the initial building blocks. The as-prepared CI-GNCs exhibit highly crystalline graphitic nanostructures. Moreover, they possess promising electrocatalytic activity for the oxygen reaction reduction (ORR) in alkaline medium. This simple fabrication technology presents a great advance for synthesizing CI-GNCs composite catalysts, which have potential as new metal-free catalysts for efficient ORR applications.

KW - carbon

KW - electrocatalysis

KW - graphene quantum dots

KW - graphite nanocapsules

KW - oxygen reduction reaction

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Unusual Assembly and Conversion of Graphene Quantum Dots into Crystalline Graphite Nanocapsules

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