Stabilization and Emission Characteristics of Gliding Arc-Assisted NH3/CH4/Air Premixed Flames in a Swirl Combustor

Jinguo Sun, Qian Huang, Yong Tang, Shuiqing Li*

*此作品的通讯作者

科研成果: 期刊稿件文章同行评审

16 引用 (Scopus)

摘要

This paper investigates the effects of gliding arc (GA) discharge on the stabilization and emission characteristics of premixed NH3/CH4/air swirl flames under various ammonia contents, flow rates, and global equivalence ratios. First, the lean blowout (LBO) limits are measured. We find that although blending CH4extends the LBO limit of the ammonia flame to 0.6-0.8, the GA discharge further remarkably extends it to 0.3-0.4. Then, the flow and flame structures are visualized by simultaneous OH planar laser-induced fluorescence and particle imaging velocimetry measurements. The results reveal that the discharge increases the OH radical concentration and expands the inner recirculation zone, leading to improved flame stability. Second, the NOxemissions are investigated over a wide range of global equivalence ratios and ammonia contents. It is seen that the GA discharge slightly increases the NOxemission by less than 7% at low NH3contents (<0.6), which can be attributed to the thermal and OH-involved reaction pathway of NOxformation. However, as the NH3content further increases (which is accompanied by the rapid growth of the NOxemission), the GA discharge effectively reduces the NOxemission by up to 30%. This effect might be due to the more intensive NOx-consuming reactions by plasma-induced NH2radicals at a higher ammonia content, which is confirmed by the strengthened NH2∗ chemiluminescence under GA discharge conditions. Finally, a chemical reactor network analysis gives reasonable NOxpredictions without GA discharge and highlights the NOx-reduction effects of NH2radicals under high ammonia contents.

源语言英语
页(从-至)8520-8527
页数8
期刊Energy and Fuels
36
15
DOI
出版状态已出版 - 4 8月 2022

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