Identification of Atomic Defects and Adsorbate on Rutile TiO2(110)-(1 × 1) Surface by Atomic Force Microscopy

Huan Fei Wen, Yuuki Adachi, Quanzhen Zhang, Masato Miyazaki, Yasuhiro Sugawara, Yan Jun Li*

*此作品的通讯作者

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15 引用 (Scopus)

摘要

Atomic force microscopy (AFM) has been developed as a powerful tool to study surface topography and surface chemistry with atomic resolution, whereas straightforward identification of surface point defect/adsorbate is far from trivial in AFM imaging due to its complex mechanism. In this work, we successfully demonstrate a reliable way to discriminate surface point defect/adsorbate on a rutile TiO2 surface by AFM. Each surface point defect/adsorbate can positively respond to the applied bias voltage, but the specific response value is different. The present methodology is reliable to distinguish the surface atomic defect and adsorbates on metal oxides, no matter what kinds of tip apex termination, and useful for continuous investigation of catalytic reactions on the surface.

源语言英语
页(从-至)25756-25760
页数5
期刊Journal of Physical Chemistry C
123
42
DOI
出版状态已出版 - 24 10月 2019
已对外发布

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Wen, H. F., Adachi, Y., Zhang, Q., Miyazaki, M., Sugawara, Y., & Li, Y. J. (2019). Identification of Atomic Defects and Adsorbate on Rutile TiO2(110)-(1 × 1) Surface by Atomic Force Microscopy. Journal of Physical Chemistry C, 123(42), 25756-25760. https://doi.org/10.1021/acs.jpcc.9b07949