Chiral Squaramide Catalyzed Asymmetric [3+2] Cycloaddition Reaction for Synthesis of Trifluoromethylated Barbituric Acid Derivatives

Tian Li An, Da Ming Du*

*此作品的通讯作者

科研成果: 期刊稿件文章同行评审

18 引用 (Scopus)

摘要

A squaramide catalyzed asymmetric Michael/Mannich [3+2] cycloaddition reaction between N-2,2,2-trifluoroethyl isatin ketimines and barbiturate-based olefins was developed. The corresponding trifluoromethylated dispirobarbituric acid derivatives containing three stereocenters were obtained in excellent yields and stereoselectivities (up to 99% yield, 99:1 dr and >99% ee). In addition, the gram-scale reaction also achieved with excellent yield and stereoselectivity.

源语言英语
页(从-至)11302-11306
页数5
期刊ChemistrySelect
4
38
DOI
出版状态已出版 - 17 10月 2019

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