Experimental Evidence of Chiral Symmetry Breaking in Kekulé-Ordered Graphene

Changhua Bao, Hongyun Zhang, Teng Zhang, Xi Wu, Laipeng Luo, Shaohua Zhou, Qian Li, Yanhui Hou, Wei Yao, Liwei Liu, Pu Yu, Jia Li, Wenhui Duan, Hong Yao, Yeliang Wang, Shuyun Zhou*

*Corresponding author for this work

Research output: Contribution to journalArticlepeer-review

80 Citations (Scopus)

Abstract

The low-energy excitations of graphene are relativistic massless Dirac fermions with opposite chiralities at valleys K and K′. Breaking the chiral symmetry could lead to gap opening in analogy to dynamical mass generation in particle physics. Here we report direct experimental evidences of chiral symmetry breaking (CSB) from both microscopic and spectroscopic measurements in a Li-intercalated graphene. The CSB is evidenced by gap opening at the Dirac point, Kekulé-O type modulation, and chirality mixing near the gap edge. Our work opens up opportunities for investigating CSB related physics in a Kekulé-ordered graphene.

Original languageEnglish
Article number206804
JournalPhysical Review Letters
Volume126
Issue number20
DOIs
Publication statusPublished - 19 May 2021

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