TiO2-anchored three-dimensional integration of layer covalent organic framework for photocatalytic H2 production

Ai Juan Li; Tao Zhang; Sheng Li Huang

doi:10.1016/j.apcata.2024.120068

TiO₂-anchored three-dimensional integration of layer covalent organic framework for photocatalytic H₂ production

Ai Juan Li, Tao Zhang, Sheng Li Huang^*

^*此作品的通讯作者

化学与化工学院

Beijing Institute of Technology

科研成果: 期刊稿件 › 文章 › 同行评审

摘要

Photocatalytic H₂ production presents great significance for sustainable development of energy and economy. Covalent organic frameworks (COFs) have received huge attention in photocatalytic applications. Herein, crystalline OH-COFs were synthesized through the transformation of imine bond to quinoline ring via Povarov reaction. TiO₂-COF exhibited excellent photocatalytic performance for H₂ production in H₂O/alcohol system. This strategy provides available method for the design and synthesis of highly efficient photocatalysts based on COF-inorganic semiconductor hybridization.

源语言	英语
文章编号	120068
期刊	Applied Catalysis A: General
卷	691
DOI	https://doi.org/10.1016/j.apcata.2024.120068
出版状态	已出版 - 5 2月 2025

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10.1016/j.apcata.2024.120068

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title = "TiO2-anchored three-dimensional integration of layer covalent organic framework for photocatalytic H2 production",

abstract = "Photocatalytic H2 production presents great significance for sustainable development of energy and economy. Covalent organic frameworks (COFs) have received huge attention in photocatalytic applications. Herein, crystalline OH-COFs were synthesized through the transformation of imine bond to quinoline ring via Povarov reaction. TiO2-COF exhibited excellent photocatalytic performance for H2 production in H2O/alcohol system. This strategy provides available method for the design and synthesis of highly efficient photocatalysts based on COF-inorganic semiconductor hybridization.",

keywords = "Hybridization, Photocatalytic H production, Quinoline COFs, TiO",

author = "Li, {Ai Juan} and Tao Zhang and Huang, {Sheng Li}",

note = "Publisher Copyright: {\textcopyright} 2024",

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doi = "10.1016/j.apcata.2024.120068",

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AU - Li, Ai Juan

AU - Zhang, Tao

AU - Huang, Sheng Li

PY - 2025/2/5

Y1 - 2025/2/5

N2 - Photocatalytic H2 production presents great significance for sustainable development of energy and economy. Covalent organic frameworks (COFs) have received huge attention in photocatalytic applications. Herein, crystalline OH-COFs were synthesized through the transformation of imine bond to quinoline ring via Povarov reaction. TiO2-COF exhibited excellent photocatalytic performance for H2 production in H2O/alcohol system. This strategy provides available method for the design and synthesis of highly efficient photocatalysts based on COF-inorganic semiconductor hybridization.

AB - Photocatalytic H2 production presents great significance for sustainable development of energy and economy. Covalent organic frameworks (COFs) have received huge attention in photocatalytic applications. Herein, crystalline OH-COFs were synthesized through the transformation of imine bond to quinoline ring via Povarov reaction. TiO2-COF exhibited excellent photocatalytic performance for H2 production in H2O/alcohol system. This strategy provides available method for the design and synthesis of highly efficient photocatalysts based on COF-inorganic semiconductor hybridization.

KW - Hybridization

KW - Photocatalytic H production

KW - Quinoline COFs

KW - TiO

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JO - Applied Catalysis A: General

JF - Applied Catalysis A: General

M1 - 120068

ER -

TiO2-anchored three-dimensional integration of layer covalent organic framework for photocatalytic H2 production

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TiO₂-anchored three-dimensional integration of layer covalent organic framework for photocatalytic H₂ production