Surface plasmon enhanced exciton transitions, cavity resonance effects, and exciton-/polariton-LO phonon interactions in ZnO nanowires

Duan Zhao, Gangbei Zhu, Yongyou Zhang*, Yanchun Wang, Weiya Zhou, Sishen Xie*, Bingsuo Zou*

*此作品的通讯作者

科研成果: 期刊稿件文章同行评审

3 引用 (Scopus)

摘要

Optical properties of single-subwavelength ZnO nanowires are highly improved by the Al2O3 layer/rough Ag film plasmonic structure as a substrate, owing to the exciton-surface plasmon (SP) interactions. The ZnO nanowire luminescence efficiency was enhanced on the Al2O3 layer/rough Ag film as compared with the SiO2/Si substrate. The exciton transitions can be highly enhanced with narrow linewidth and distinguished clearly above 80 K. Typically, three different bound exciton transitions originating from different impurities as trap centers can be identified at 80 K and traced clearly before thermal dissociation. Meanwhile, the strong local electromagnetic field induced by SP can enhance the whispering-gallery-mode (WGM) resonance and the exciton-/exciton-polariton (polariton for short)-longitudinal optical (LO) phonon interaction. The formation of WGM polaritons with energy in the region of first-order LO phonon replica is efficiently promoted by polariton-LO phonon scattering relaxation. These findings provide an effective method for designing novel semiconductor-nanostructure luminescence or lasing devices in future.

源语言英语
页(从-至)28252-28260
页数9
期刊Journal of Physical Chemistry C
124
51
DOI
出版状态已出版 - 24 12月 2020

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