TY - JOUR
T1 - Repeatedly and Superbroad Wavelength Tuning Microcavity in a Single Sn-Doped CdS Microcone
AU - Tian, Ye
AU - Peng, Hui
AU - Yao, Shangfei
AU - Zhou, Zhijie
AU - Ke, Bao
AU - Lin, Wenchao
AU - Lu, Fuxi
AU - Yu, Zongmian
AU - Jia, Wenyong
AU - Zhang, Yongyou
AU - Zou, Bingsuo
N1 - Publisher Copyright:
© 2022 American Chemical Society. All rights reserved.
PY - 2022/8/4
Y1 - 2022/8/4
N2 - It is a challenge to realize the mode wavelength tunability of microcavity in a wide spectral range but critically important for the practical application of optoelectronic devices. Here, we report a Sn-doped CdS microcone with tunable microcavity properties, and the tuning range is more than 300 nm, which is the largest tunable range in a single nanostructure. Its photoluminescence (PL) mapping showed the existence of the periodic structure in the Sn-doped CdS microcone and the selection propagation of longitudinal photons. Cross-sectional radius-dependent PL spectra show a continuous transition from a multimode to three-mode microcavity with decreasing cross-section radius, which indicates the character of different whisper-gallery mode (WGM) microcavity. Meanwhile, the calculation shows that the plane-wave model allows a good description of the detected spectral profile. Our approach simultaneously achieves both wide-spectra and repeatably adjustable microcavity in a single nanostructure. This nanostructure provides a new platform to study wavelength controllability-related high-performance photoelectric detection.
AB - It is a challenge to realize the mode wavelength tunability of microcavity in a wide spectral range but critically important for the practical application of optoelectronic devices. Here, we report a Sn-doped CdS microcone with tunable microcavity properties, and the tuning range is more than 300 nm, which is the largest tunable range in a single nanostructure. Its photoluminescence (PL) mapping showed the existence of the periodic structure in the Sn-doped CdS microcone and the selection propagation of longitudinal photons. Cross-sectional radius-dependent PL spectra show a continuous transition from a multimode to three-mode microcavity with decreasing cross-section radius, which indicates the character of different whisper-gallery mode (WGM) microcavity. Meanwhile, the calculation shows that the plane-wave model allows a good description of the detected spectral profile. Our approach simultaneously achieves both wide-spectra and repeatably adjustable microcavity in a single nanostructure. This nanostructure provides a new platform to study wavelength controllability-related high-performance photoelectric detection.
UR - http://www.scopus.com/inward/record.url?scp=85136132677&partnerID=8YFLogxK
U2 - 10.1021/acs.jpcc.2c04142
DO - 10.1021/acs.jpcc.2c04142
M3 - Article
AN - SCOPUS:85136132677
SN - 1932-7447
VL - 126
SP - 12696
EP - 12703
JO - Journal of Physical Chemistry C
JF - Journal of Physical Chemistry C
IS - 30
ER -