TY - JOUR
T1 - Regulation of 2D Graphene Materials for Electrocatalysis
AU - Zhang, Xinqun
AU - Gao, Jian
AU - Xiao, Yukun
AU - Wang, Jiaqi
AU - Sun, Guoqiang
AU - Zhao, Yang
AU - Qu, Liangti
N1 - Publisher Copyright:
© 2020 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim
PY - 2020/8/3
Y1 - 2020/8/3
N2 - Benefiting from unique excellent physical and chemical characteristics, graphene has attracted widespread attention in the application of electrocatalysis. As a promising candidate, graphene is usually regulated with surface defects, heteroatoms, metal atoms and other active materials through covalent or non-covalent bonds to substitute for noble metal catalysts, which has not been targeted in a report yet. In this review, we summarize the recent advances of approaches for engineering graphene-based electrocatalysts and emphasize the corresponding electrocatalytic active sites in various electrocatalysis circumstances, such as electrocatalytic hydrogen evolution reaction (HER), oxygen evolution reaction (OER), oxygen reduction reaction (ORR), etc. The opportunities and challenges in the future development of graphene-based catalysts are also discussed.
AB - Benefiting from unique excellent physical and chemical characteristics, graphene has attracted widespread attention in the application of electrocatalysis. As a promising candidate, graphene is usually regulated with surface defects, heteroatoms, metal atoms and other active materials through covalent or non-covalent bonds to substitute for noble metal catalysts, which has not been targeted in a report yet. In this review, we summarize the recent advances of approaches for engineering graphene-based electrocatalysts and emphasize the corresponding electrocatalytic active sites in various electrocatalysis circumstances, such as electrocatalytic hydrogen evolution reaction (HER), oxygen evolution reaction (OER), oxygen reduction reaction (ORR), etc. The opportunities and challenges in the future development of graphene-based catalysts are also discussed.
KW - design strategies
KW - electrocatalysts
KW - electronic properties
KW - energy conversion
KW - graphene
UR - http://www.scopus.com/inward/record.url?scp=85085105666&partnerID=8YFLogxK
U2 - 10.1002/asia.202000249
DO - 10.1002/asia.202000249
M3 - Review article
C2 - 32227581
AN - SCOPUS:85085105666
SN - 1861-4728
VL - 15
SP - 2271
EP - 2281
JO - Chemistry - An Asian Journal
JF - Chemistry - An Asian Journal
IS - 15
ER -