Regulating the electronic structure of manganese-based materials to optimize the performance of zinc-ion batteries

Anqi Zhang, Ran Zhao*, Yahui Wang, Jing Jing Yang, Chuan Wu*, Ying Bai*

*此作品的通讯作者

科研成果: 期刊稿件文献综述同行评审

67 引用 (Scopus)

摘要

Manganese-based materials are considered as one of the most promising energy storage cathode materials for zinc-ion batteries (ZIBs). To achieve major breakthroughs in commercialization, optimizing their poor inherent performance through various modification methods has attracted extensive attention. The previous reviews have mainly focused on the improvement of electrochemical performance and specific means but lack a discussion of the common internal mechanisms that various regulatory strategies can bring about significant changes in the electronic structure, which is insufficient to provide in-depth guidance and reference for electrochemical performance optimization of manganese-based materials. Herein, by summarizing the contribution of almost all modification strategies to the significant changes in the electronic structure, this review discloses that electronic structure regulation can be used as a general means to optimize the intrinsic properties and proposes a top-down electrochemical performance optimization methodology, which provides comprehensive suggestions for the optimization of manganese-based material performance. Notably, the electronic structure regulation effects of different modification methods are thoroughly compared, and their applicability and economy are evaluated, which is expected to further accelerate the commercialization of manganese-based ZIBs.

源语言英语
页(从-至)3240-3301
页数62
期刊Energy and Environmental Science
16
8
DOI
出版状态已出版 - 6 7月 2023

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Zhang, A., Zhao, R., Wang, Y., Yang, J. J., Wu, C., & Bai, Y. (2023). Regulating the electronic structure of manganese-based materials to optimize the performance of zinc-ion batteries. Energy and Environmental Science, 16(8), 3240-3301. https://doi.org/10.1039/d3ee01344h