TY - JOUR
T1 - Rational Design of MOF-Based Materials for Next-Generation Rechargeable Batteries
AU - Ye, Zhengqing
AU - Jiang, Ying
AU - Li, Li
AU - Wu, Feng
AU - Chen, Renjie
N1 - Publisher Copyright:
© 2021, The Author(s).
PY - 2021/12
Y1 - 2021/12
N2 - Metal–organic framework (MOF)-based materials with high porosity, tunable compositions, diverse structures, and versatile functionalities provide great scope for next-generation rechargeable battery applications. Herein, this review summarizes recent advances in pristine MOFs, MOF composites, MOF derivatives, and MOF composite derivatives for high-performance sodium-ion batteries, potassium-ion batteries, Zn-ion batteries, lithium–sulfur batteries, lithium–oxygen batteries, and Zn–air batteries in which the unique roles of MOFs as electrodes, separators, and even electrolyte are highlighted. Furthermore, through the discussion of MOF-based materials in each battery system, the key principles for controllable synthesis of diverse MOF-based materials and electrochemical performance improvement mechanisms are discussed in detail. Finally, the major challenges and perspectives of MOFs are also proposed for next-generation battery applications.[Figure not available: see fulltext.].
AB - Metal–organic framework (MOF)-based materials with high porosity, tunable compositions, diverse structures, and versatile functionalities provide great scope for next-generation rechargeable battery applications. Herein, this review summarizes recent advances in pristine MOFs, MOF composites, MOF derivatives, and MOF composite derivatives for high-performance sodium-ion batteries, potassium-ion batteries, Zn-ion batteries, lithium–sulfur batteries, lithium–oxygen batteries, and Zn–air batteries in which the unique roles of MOFs as electrodes, separators, and even electrolyte are highlighted. Furthermore, through the discussion of MOF-based materials in each battery system, the key principles for controllable synthesis of diverse MOF-based materials and electrochemical performance improvement mechanisms are discussed in detail. Finally, the major challenges and perspectives of MOFs are also proposed for next-generation battery applications.[Figure not available: see fulltext.].
KW - Batteries
KW - MOF composite derivatives
KW - MOF composites
KW - MOF derivatives
KW - Metal–organic frameworks
UR - http://www.scopus.com/inward/record.url?scp=85116372137&partnerID=8YFLogxK
U2 - 10.1007/s40820-021-00726-z
DO - 10.1007/s40820-021-00726-z
M3 - Review article
AN - SCOPUS:85116372137
SN - 2311-6706
VL - 13
JO - Nano-Micro Letters
JF - Nano-Micro Letters
IS - 1
M1 - 203
ER -