Osmapyridine and Osmapyridinium from a formal [4+2] cycloaddition reaction

Bin Liu, Huijuan Wang, Hujun Xie, Birong Zeng, Jinxiang Chen, Jun Tao, Ting Bin Wen, Zexing Cao, Haiping Xia*

*此作品的通讯作者

科研成果: 期刊稿件文章同行评审

87 引用 (Scopus)

摘要

Metalla-cycloaddition: An unprecedented formal [4+2] cycloaddition reaction takes place when osmium hydrido alkenylcarbyne 1 reacts with acetonitrile to afford the first metallapyridinium complex 2 in high yield (see scheme). Deprotonation of 2 gives the first osmapyridine compound 3. Treatment of 3 with HBF4 can regenerate 2 in almost quantitative yield.

源语言英语
页(从-至)5430-5434
页数5
期刊Angewandte Chemie - International Edition
48
30
DOI
出版状态已出版 - 13 7月 2009
已对外发布

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