One-pot synthesis of Cu:InP multishell quantum dots for near-infrared light-emitting devices

Pan Huang, Xiaonan Liu, Xiao Liu, Jing Wei, Fangze Liu*, Hongbo Li*

*此作品的通讯作者

科研成果: 期刊稿件文章同行评审

摘要

InP quantum dots (QDs) are promising heavy-metal-free materials for next-generation solid-state lighting, covering from visible to near-infrared (NIR) range. Compared with the rapid development of visible InP QDs, the synthesis of high-performance NIR InP QDs remains to be solved. In this work, we report a simple one-pot synthesis of NIR InP QDs by controlling the Cu doping and designing a multishell structure. By replacing the conventional highly reactive phosphorus precursor with a slightly less reactive and low-cost ammonia phosphorus precursor, the nucleation process is effectively regulated for efficient Cu doping. In addition, the epitaxial growth of the ZnSe/ZnS shell further improves the stability and optical properties of InP QDs. Therefore, the synthesized Cu:InP/ZnSe/ZnS QDs have a photoluminescence quantum yield of 70% centered at 833 nm. The NIR InP light-emitting diodes exhibit a maximum radiance of 3.1 W·sr−1·m−2 and a peak external quantum efficiency of 2.71% centered at 864 nm. (Figure presented.)

源语言英语
期刊Nano Research
DOI
出版状态已接受/待刊 - 2024

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