Observation of Photodielectric Effect in Aluminum Nitride Piezoelectric Films

Huiqian Yang, Jing Sun, Zaheen Uddin, Gongtian Chen, Sanxia Yin, Shengwen Liu, Tingjun Wang, Shaoqing Xu, Shulin Chen, Jian Zhou, Hang Luo, Dou Zhang, Jiawang Hong, Bin Yang*

*此作品的通讯作者

科研成果: 期刊稿件文章同行评审

1 引用 (Scopus)

摘要

Piezoelectric semiconductors hold great promise for the development of optoelectronic devices due to the presence of a photodielectric effect (PDE), which has been observed in perovskite ferroelectric ceramics. However, the PDE in wurtzite-structured aluminum nitride (AlN) and how light affects dielectric properties remain unexplored. Here, we observed PDE of AlN films in the low-frequency region around 20 Hz to 1 MHz. The permittivity (ϵr) increased after light irradiation, and the change in ϵr increased with larger photon energy, accompanied by an increase in dielectric loss (tan δ). For Sc0.15Al0.85N, the change in Δϵ was significantly larger compared to AlN, whereas the variation of tan δ became smaller. The PDE exhibited reversible light-induced switching of piezoelectric polarization, and the time required for ϵr to saturate under light illumination was shorter for Sc0.15Al0.85N than AlN. This work provides a fundamental understanding for photocontrolled piezoelectric properties for exploration of better piezoelectric semiconductors with photodielectric behavior.

源语言英语
期刊ACS Applied Electronic Materials
DOI
出版状态已接受/待刊 - 2024

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