Local Plastic Response and Slow Heterogeneous Dynamics of Supercooled Liquids

Yan Wei Li, Yugui Yao, Massimo Pica Ciamarra

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摘要

We demonstrate, via numerical simulations, that the relaxation dynamics of supercooled liquids correlates well with a plastic length scale measuring a particle's response to impulsive localized perturbations and weakly to measures of local elasticity. We find that the particle averaged plastic length scale vanishes linearly in temperature and controls the super-Arrhenius temperature dependence of the relaxation time. Furthermore, we show that the plastic length scale of individual particles correlates with their typical displacement at the relaxation time. In contrast, the local elastic response only correlates with the dynamics on the vibrational timescale.

源语言英语
文章编号258001
期刊Physical Review Letters
128
25
DOI
出版状态已出版 - 24 6月 2022

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Li, Y. W., Yao, Y., & Ciamarra, M. P. (2022). Local Plastic Response and Slow Heterogeneous Dynamics of Supercooled Liquids. Physical Review Letters, 128(25), 文章 258001. https://doi.org/10.1103/PhysRevLett.128.258001