Investigation of double-pulse femtosecond laser induced breakdown spectroscopy of polymethyl methacrylate (PMMA)

Mengmeng Wang, Sumei Wang, Zhitao Cao, Peng Wang, Cong Wangc

科研成果: 书/报告/会议事项章节会议稿件同行评审

9 引用 (Scopus)

摘要

The emission properties of double-pulse (DP) over single-pulse (SP) femtosecond laser breakdown spectroscopy (fs-LIBS) of polymethyl methacrylate (PMMA) were investigated. The signal enhancements in the DP fs-LIBS strongly depended on the DP delay and were influenced by the type of emission particles. Intensity enhancement of emission lines increased in the sequence of molecules, neutral atoms, and ions. Electron density and temperature were reported to characterize the plasmas. Both the electron density and plasma temperature exhibit similar variation trajectories with respect to the DP delay and feature a distinct increase at an optimal DP delay of ∼80 ps, indicating reheating of preproduced plume is responsible for the emission enhancement. The dependence of the signal emission on laser energy was also studied, showing the emission intensity was linear to the pulse energy. However, the signal enhancement was nonlinear to the pulse energy, suggesting that the signal enhancement was related to the energy coupling efficiency of second pulse to the first pulse generated plume.

源语言英语
主期刊名Laser-Based Micro- and Nanoprocessing IX
编辑Udo Klotzbach, Kunihiko Washio, Craig B. Arnold
出版商SPIE
ISBN(电子版)9781628414417
DOI
出版状态已出版 - 2015
活动Laser-Based Micro- and Nanoprocessing IX - San Francisco, 美国
期限: 10 2月 201512 2月 2015

出版系列

姓名Proceedings of SPIE - The International Society for Optical Engineering
9351
ISSN(印刷版)0277-786X
ISSN(电子版)1996-756X

会议

会议Laser-Based Micro- and Nanoprocessing IX
国家/地区美国
San Francisco
时期10/02/1512/02/15

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