TY - JOUR
T1 - High-Efficient Anti-Icing/Deicing Method Based on Graphene Foams
AU - Huang, Jianan
AU - Li, Dawei
AU - Peng, Zhilong
AU - Zhang, Bo
AU - Yao, Yin
AU - Chen, Shaohua
N1 - Publisher Copyright:
© 2023 American Chemical Society.
PY - 2023/9/13
Y1 - 2023/9/13
N2 - Anti-icing/deicing has always been a focal issue in modern industries. A novel anti-icing/deicing material based on graphene foams (GF) is prepared in this paper, which integrates multiple functions, including electrothermal conversion, photothermal conversion, and superhydrophobicity. The GF sheet is used as a bottom layer bonded on the protected substrate, which is covered by a polymeric composite coating filled with TiN and SiO2 nanoparticles. Electric heating and light heating experiments are performed to study the anti-icing/deicing performances of such a GF-based material. It is found that, under the unique action of electric fields, a voltage of only 1 V is needed to increase the surface temperature from minus tens of degrees to the one above zero within 400 s, which is much lower than their previous counterparts of more than 10 V to achieve the same unfreezing effect. A slight increase of the applied voltage to 1.5 V can even result in a remarkable increase of the surface temperature from room temperature to more than 150 °C within 200 s, in contrast to existing electric heating techniques to attain peak temperatures of about 100 °C at the expense of tens of volts. Such performances enable the GF-based material to achieve an outstanding electrothermal energy conversion rate of more than 90%. Furthermore, with the help of sunlight illumination in addition to the electric power, not only can the critical voltage to prevent icing be reduced but also a much more rapid and adequate removal of ice or frost from the surface can be realized compared with the deicing/defrosting performance under either electric or light field alone. All of these results demonstrate the obvious advantages of the present method in superior energy utilization efficiency and universal applicability to dark and sunlight environments, which should be particularly useful for at-all-cost protection of key components in industrial equipment from icing.
AB - Anti-icing/deicing has always been a focal issue in modern industries. A novel anti-icing/deicing material based on graphene foams (GF) is prepared in this paper, which integrates multiple functions, including electrothermal conversion, photothermal conversion, and superhydrophobicity. The GF sheet is used as a bottom layer bonded on the protected substrate, which is covered by a polymeric composite coating filled with TiN and SiO2 nanoparticles. Electric heating and light heating experiments are performed to study the anti-icing/deicing performances of such a GF-based material. It is found that, under the unique action of electric fields, a voltage of only 1 V is needed to increase the surface temperature from minus tens of degrees to the one above zero within 400 s, which is much lower than their previous counterparts of more than 10 V to achieve the same unfreezing effect. A slight increase of the applied voltage to 1.5 V can even result in a remarkable increase of the surface temperature from room temperature to more than 150 °C within 200 s, in contrast to existing electric heating techniques to attain peak temperatures of about 100 °C at the expense of tens of volts. Such performances enable the GF-based material to achieve an outstanding electrothermal energy conversion rate of more than 90%. Furthermore, with the help of sunlight illumination in addition to the electric power, not only can the critical voltage to prevent icing be reduced but also a much more rapid and adequate removal of ice or frost from the surface can be realized compared with the deicing/defrosting performance under either electric or light field alone. All of these results demonstrate the obvious advantages of the present method in superior energy utilization efficiency and universal applicability to dark and sunlight environments, which should be particularly useful for at-all-cost protection of key components in industrial equipment from icing.
KW - anti-icing/deicing method
KW - electrothermal conversion
KW - energy utilization efficiency
KW - graphene foam (GF)
KW - photothermal conversion
UR - http://www.scopus.com/inward/record.url?scp=85171203392&partnerID=8YFLogxK
U2 - 10.1021/acsami.3c09360
DO - 10.1021/acsami.3c09360
M3 - Article
C2 - 37647497
AN - SCOPUS:85171203392
SN - 1944-8244
VL - 15
SP - 43026
EP - 43037
JO - ACS applied materials & interfaces
JF - ACS applied materials & interfaces
IS - 36
ER -