Helicity resolved ultrafast pump-probe spectroscopy of monolayer molybdenum disulphide

Jun Qiu, Qinsheng Wang, Shaofeng Ge, Yanxin Ji, Dong Sun*

*此作品的通讯作者

科研成果: 书/报告/会议事项章节会议稿件同行评审

摘要

We investigate the valley related carrier dynamics in monolayer MoS2 using helicity resolved non-degenerate ultrafast pump-probe spectroscopy at the vicinity of the high-symmetry K point under the temperature down to 78 K. Monolayer MoS2 shows remarkable transient reflection signals, in stark contrast to bilayer and bulk MoS2 due to the enhancement of many-body effect at reduced dimensionality. The helicity resolved ultrafast time-resolved result shows that the valley polarization is preserved for only several ps before scattering process makes it undistinguishable. We suggest that the dynamical degradation of valley polarization is attributable primarily to the exciton trapping by defect states in the exfoliated MoS2 samples.

源语言英语
主期刊名Ultrafast Nonlinear Imaging and Spectroscopy II
编辑Iam Choon Khoo, Zhiwen Liu, Demetri Psaltis
出版商SPIE
ISBN(电子版)9781628412253
DOI
出版状态已出版 - 2014
已对外发布
活动Ultrafast Nonlinear Imaging and Spectroscopy II - San Diego, 美国
期限: 17 8月 201418 8月 2014

出版系列

姓名Proceedings of SPIE - The International Society for Optical Engineering
9198
ISSN(印刷版)0277-786X
ISSN(电子版)1996-756X

会议

会议Ultrafast Nonlinear Imaging and Spectroscopy II
国家/地区美国
San Diego
时期17/08/1418/08/14

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