Enantioselective Addition of Pyrazoles to Dienes**

Alexander Y. Jiu, Hannah S. Slocumb, Charles S. Yeung, Xiao Hui Yang*, Vy M. Dong*

*此作品的通讯作者

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69 引用 (Scopus)

摘要

We report the first enantioselective addition of pyrazoles to 1,3-dienes. Secondary and tertiary allylic pyrazoles can be generated with excellent regioselectivity. Mechanistic studies support a pathway distinct from previous hydroaminations: a Pd0-catalyzed ligand-to-ligand hydrogen transfer (LLHT). This hydroamination tolerates a range of functional groups and advances the field of diene hydrofunctionalization.

源语言英语
页(从-至)19660-19664
页数5
期刊Angewandte Chemie - International Edition
60
36
DOI
出版状态已出版 - 1 9月 2021

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