Dominant role of emission reduction in PM2.5 air quality improvement in Beijing during 2013-2017: A model-based decomposition analysis

In 2013, China's government published the Air Pollution Prevention and Control Action Plan (APPCAP) with a specific target for Beijing, which aims to reduce annual mean PM<span classCombining double low line"inline-formula">2.5</span> concentrations in Beijing to 60&thinsp;<span classCombining double low line"inline-formula">μ</span>g&thinsp;m<span classCombining double low line"inline-formula">-3</span> in 2017. During 2013-2017, the air quality in Beijing was significantly improved following the implementation of various emission control measures locally and regionally, with the annual mean PM<span classCombining double low line"inline-formula">2.5</span> concentration decreasing from 89.5&thinsp;<span classCombining double low line"inline-formula">μ</span>g&thinsp;m<span classCombining double low line"inline-formula">-3</span> in 2013 to 58&thinsp;<span classCombining double low line"inline-formula">μ</span>g&thinsp;m<span classCombining double low line"inline-formula">-3</span> in 2017. As meteorological conditions were more favourable to the reduction of air pollution in 2017 than in 2013 and 2016, the real effectiveness of emission control measures on the improvement of air quality in Beijing has frequently been questioned.

In this work, by combining a detailed bottom-up emission inventory over Beijing, the MEIC regional emission inventory and the WRF-CMAQ (Weather Research and Forecasting Model and Community Multiscale Air Quality) model, we attribute the improvement in Beijing's PM<span classCombining double low line"inline-formula">2.5</span> air quality in 2017 (compared to 2013 and 2016) to the following factors: changes in meteorological conditions, reduction of emissions from surrounding regions, and seven specific categories of local emission control measures in Beijing. We collect and summarize data related to 32 detailed control measures implemented during 2013-2017, quantify the emission reductions associated with each measure using the bottom-up local emission inventory in 2013, aggregate the measures into seven categories, and conduct a series of CMAQ simulations to quantify the contribution of different factors to the PM<span classCombining double low line"inline-formula">2.5</span> changes.

<span idCombining double low line"page6126"/>We found that, although changes in meteorological conditions partly explain the improved PM<span classCombining double low line"inline-formula">2.5</span> air quality in Beijing in 2017 compared to 2013 (3.8&thinsp;<span classCombining double low line"inline-formula">μ</span>g&thinsp;m<span classCombining double low line"inline-formula">-3</span>, 12.1&thinsp;% of total), the rapid decrease in PM<span classCombining double low line"inline-formula">2.5</span> concentrations in Beijing during 2013-2017 was dominated by local (20.6&thinsp;<span classCombining double low line"inline-formula">μ</span>g&thinsp;m<span classCombining double low line"inline-formula">-3</span>, 65.4&thinsp;%) and regional (7.1&thinsp;<span classCombining double low line"inline-formula">μ</span>g&thinsp;m<span classCombining double low line"inline-formula">-3</span>, 22.5&thinsp;%) emission reductions. The seven categories of emission control measures, i.e. coal-fired boiler control, clean fuels in the residential sector, optimize industrial structure, fugitive dust control, vehicle emission control, improved end-of-pipe control, and integrated treatment of VOCs, reduced the PM<span classCombining double low line"inline-formula">2.5</span> concentrations in Beijing by 5.9, 5.3, 3.2, 2.3, 1.9, 1.8, and 0.2&thinsp;<span classCombining double low line"inline-formula">μ</span>g&thinsp;m<span classCombining double low line"inline-formula">-3</span>, respectively, during 2013-2017. We also found that changes in meteorological conditions could explain roughly 30&thinsp;% of total reduction in PM<span classCombining double low line"inline-formula">2.5</span> concentration during 2016-2017 with more prominent contribution in winter months (November and December). If the meteorological conditions in 2017 had remained the same as those in 2016, the annual mean PM<span classCombining double low line"inline-formula">2.5</span> concentrations would have increased from 58 to 63&thinsp;<span classCombining double low line"inline-formula">μ</span>g&thinsp;m<span classCombining double low line"inline-formula">-3</span>, exceeding the target established in the APPCAP. Despite the remarkable impacts from meteorological condition changes, local and regional emission reductions still played major roles in the PM<span classCombining double low line"inline-formula">2.5</span> decrease in Beijing during 2016-2017, and clean fuels in the residential sector, coal-fired boiler control, and optimize industrial structure were the three most effective local measures (contributing reductions of 2.1, 1.9, and 1.5&thinsp;<span classCombining double low line"inline-formula">μ</span>g&thinsp;m<span classCombining double low line"inline-formula">-3</span>, respectively). Our study confirms the effectiveness of clean air actions in Beijing and its surrounding regions and reveals that a new generation of control measures and strengthened regional joint emission control measures should be implemented for continued air quality improvement in Beijing because the major emitting sources have changed since the implementation of the clean air actions.

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