Yang, N., Zhu, C., Chen, Y., Zai, H., Wang, C., Wang, X., Wang, H., Ma, S., Gao, Z., Wang, X., Hong, J., Bai, Y., Zhou, H., Cui, B. B., & Chen, Q. (2020). An: In situ cross-linked 1D/3D perovskite heterostructure improves the stability of hybrid perovskite solar cells for over 3000 h operation. Energy and Environmental Science, 13(11), 4344-4352. https://doi.org/10.1039/d0ee01736a
Yang, Ning ; Zhu, Cheng ; Chen, Yihua 等. / An : In situ cross-linked 1D/3D perovskite heterostructure improves the stability of hybrid perovskite solar cells for over 3000 h operation. 在: Energy and Environmental Science. 2020 ; 卷 13, 号码 11. 页码 4344-4352.
@article{1495e075addc4f7cb07b5d9d01530051,
title = "An: In situ cross-linked 1D/3D perovskite heterostructure improves the stability of hybrid perovskite solar cells for over 3000 h operation",
abstract = "Long-term stability is an essential requirement for perovskite solar cells (PSCs) to be commercially viable. Heterojunctions built by low-dimensional and three-dimensional perovskites (1D/3D or 2D/3D) help to improve the stability of PSCs. However, the insulated organic cations of low-dimensional perovskite impede the transport of carriers, decreasing the power conversion efficiency (PCE) of PSCs. Herein, we introduce an in situ cross-linking polymerizable propargylammonium (PA+) to the 3D perovskite film at surfaces and grain boundaries to form a 1D/3D perovskite heterostructure. This passivation strategy not only significantly improves the interfacial carrier transport but also releases residual tensile strain in perovskite films. As a result, the corresponding devices achieve a champion PCE of 21.19%, while maintaining 93% of their initial efficiency after 3055 h of continuous illumination under maximum power point (MPP) operating conditions.",
author = "Ning Yang and Cheng Zhu and Yihua Chen and Huachao Zai and Chenyue Wang and Xi Wang and Hao Wang and Sai Ma and Ziyan Gao and Xueyun Wang and Jiawang Hong and Yang Bai and Huanping Zhou and Cui, {Bin Bin} and Qi Chen",
note = "Publisher Copyright: {\textcopyright} The Royal Society of Chemistry.",
year = "2020",
month = nov,
doi = "10.1039/d0ee01736a",
language = "English",
volume = "13",
pages = "4344--4352",
journal = "Energy and Environmental Science",
issn = "1754-5692",
publisher = "Royal Society of Chemistry",
number = "11",
}
Yang, N, Zhu, C, Chen, Y, Zai, H, Wang, C, Wang, X, Wang, H, Ma, S, Gao, Z, Wang, X, Hong, J, Bai, Y, Zhou, H, Cui, BB & Chen, Q 2020, 'An: In situ cross-linked 1D/3D perovskite heterostructure improves the stability of hybrid perovskite solar cells for over 3000 h operation', Energy and Environmental Science, 卷 13, 号码 11, 页码 4344-4352. https://doi.org/10.1039/d0ee01736a
An: In situ cross-linked 1D/3D perovskite heterostructure improves the stability of hybrid perovskite solar cells for over 3000 h operation. / Yang, Ning
; Zhu, Cheng; Chen, Yihua 等.
在:
Energy and Environmental Science, 卷 13, 号码 11, 11.2020, 页码 4344-4352.
科研成果: 期刊稿件 › 文章 › 同行评审
TY - JOUR
T1 - An
T2 - In situ cross-linked 1D/3D perovskite heterostructure improves the stability of hybrid perovskite solar cells for over 3000 h operation
AU - Yang, Ning
AU - Zhu, Cheng
AU - Chen, Yihua
AU - Zai, Huachao
AU - Wang, Chenyue
AU - Wang, Xi
AU - Wang, Hao
AU - Ma, Sai
AU - Gao, Ziyan
AU - Wang, Xueyun
AU - Hong, Jiawang
AU - Bai, Yang
AU - Zhou, Huanping
AU - Cui, Bin Bin
AU - Chen, Qi
N1 - Publisher Copyright:
© The Royal Society of Chemistry.
PY - 2020/11
Y1 - 2020/11
N2 - Long-term stability is an essential requirement for perovskite solar cells (PSCs) to be commercially viable. Heterojunctions built by low-dimensional and three-dimensional perovskites (1D/3D or 2D/3D) help to improve the stability of PSCs. However, the insulated organic cations of low-dimensional perovskite impede the transport of carriers, decreasing the power conversion efficiency (PCE) of PSCs. Herein, we introduce an in situ cross-linking polymerizable propargylammonium (PA+) to the 3D perovskite film at surfaces and grain boundaries to form a 1D/3D perovskite heterostructure. This passivation strategy not only significantly improves the interfacial carrier transport but also releases residual tensile strain in perovskite films. As a result, the corresponding devices achieve a champion PCE of 21.19%, while maintaining 93% of their initial efficiency after 3055 h of continuous illumination under maximum power point (MPP) operating conditions.
AB - Long-term stability is an essential requirement for perovskite solar cells (PSCs) to be commercially viable. Heterojunctions built by low-dimensional and three-dimensional perovskites (1D/3D or 2D/3D) help to improve the stability of PSCs. However, the insulated organic cations of low-dimensional perovskite impede the transport of carriers, decreasing the power conversion efficiency (PCE) of PSCs. Herein, we introduce an in situ cross-linking polymerizable propargylammonium (PA+) to the 3D perovskite film at surfaces and grain boundaries to form a 1D/3D perovskite heterostructure. This passivation strategy not only significantly improves the interfacial carrier transport but also releases residual tensile strain in perovskite films. As a result, the corresponding devices achieve a champion PCE of 21.19%, while maintaining 93% of their initial efficiency after 3055 h of continuous illumination under maximum power point (MPP) operating conditions.
UR - http://www.scopus.com/inward/record.url?scp=85097512476&partnerID=8YFLogxK
U2 - 10.1039/d0ee01736a
DO - 10.1039/d0ee01736a
M3 - Article
AN - SCOPUS:85097512476
SN - 1754-5692
VL - 13
SP - 4344
EP - 4352
JO - Energy and Environmental Science
JF - Energy and Environmental Science
IS - 11
ER -
Yang N, Zhu C, Chen Y, Zai H, Wang C, Wang X 等. An: In situ cross-linked 1D/3D perovskite heterostructure improves the stability of hybrid perovskite solar cells for over 3000 h operation. Energy and Environmental Science. 2020 11月;13(11):4344-4352. doi: 10.1039/d0ee01736a