A Graphitic-C3N4 "seaweed" Architecture for Enhanced Hydrogen Evolution

Qing Han; Bing Wang; Yang Zhao; Chuangang Hu; Liangti Qu

doi:10.1002/anie.201504985

A Graphitic-C₃N₄ "seaweed" Architecture for Enhanced Hydrogen Evolution

Qing Han, Bing Wang, Yang Zhao, Chuangang Hu, Liangti Qu^*

^*此作品的通讯作者

化学与化工学院

Beijing Institute of Technology

科研成果: 期刊稿件 › 文章 › 同行评审

456 引用（Scopus）

摘要

A seaweed-like graphitic-C₃N₄ (g-C₃N₄ "seaweed") architecture has been prepared by direct calcination of the freeze-drying-assembled, hydrothermally treated dicyandiamide fiber network. The seaweed network of mesoporous g-C₃N₄ nanofibers is favorable for light harvesting, charge separation and utilization of active sites, and has highly efficient photocatalytic behavior for water splitting. It exhibits a high hydrogen-evolution rate of 9900 μmol h^-1 g^-1 (thirty times higher than that of its g-C₃N₄ bulk counterpart), and a remarkable apparent quantum efficiency of 7.8 % at 420 nm, better than most of the g-C₃N₄ nanostructures reported. This work presents a very simple method for designing and developing high-performance catalysts for hydrogen evolution.

源语言	英语
页（从-至）	11433-11437
页数	5
期刊	Angewandte Chemie - International Edition
卷	54
期	39
DOI	https://doi.org/10.1002/anie.201504985
出版状态	已出版 - 1 9月 2015

联合国可持续发展目标

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10.1002/anie.201504985

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引用此

Han, Q., Wang, B., Zhao, Y., Hu, C., & Qu, L. (2015). A Graphitic-C₃N₄ "seaweed" Architecture for Enhanced Hydrogen Evolution. Angewandte Chemie - International Edition, 54(39), 11433-11437. https://doi.org/10.1002/anie.201504985

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AU - Zhao, Yang

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AU - Qu, Liangti

PY - 2015/9/1

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A Graphitic-C3N4 "seaweed" Architecture for Enhanced Hydrogen Evolution

摘要

联合国可持续发展目标

访问文件

其它文件与链接

指纹

引用此

A Graphitic-C₃N₄ "seaweed" Architecture for Enhanced Hydrogen Evolution