TY - JOUR
T1 - Visualization of Strain-Engineered Nanopattern in Center-Confined Mesoscopic WS2Monolayer Flakes
AU - Xu, Rui
AU - Lun, Yingzhuo
AU - Meng, Lan
AU - Pang, Fei
AU - Pan, Yuhao
AU - Zheng, Zhiyue
AU - Lei, Le
AU - Hussain, Sabir
AU - Li, Yan Jun
AU - Sugawara, Yasuhiro
AU - Hong, Jiawang
AU - Ji, Wei
AU - Cheng, Zhihai
N1 - Publisher Copyright:
© 2022 American Chemical Society. All rights reserved.
PY - 2022/4/28
Y1 - 2022/4/28
N2 - Strain engineering plays a crucial role in controlling the physical properties of two-dimensional (2D) materials. However, the mechanical behavior of stressed 2D crystals has not been fully understood. In this study, the fracture behavior and accompanying properties of a strained single-crystal monolayer WS2of submicron scale were investigated using a theoretical-experimental joint study. After thermal strain, the WS2monolayer was split into different forms by several cracks, with the cause of the crack formation being studied using finite element analysis (FEA). The cracks were initiated from the vertex of the nucleation center, extending along the stronger von Mises stress isolines and terminating at the edges of the monolayers. Within the separate sections, ripple regions were observed, forming several typical nanopatterns. The band gap, frictional, viscosity, and elasticity characteristics of the different strain regions were also investigated. The nanopattern should enable flexibility in the design of more sophisticated devices based on 2D materials.
AB - Strain engineering plays a crucial role in controlling the physical properties of two-dimensional (2D) materials. However, the mechanical behavior of stressed 2D crystals has not been fully understood. In this study, the fracture behavior and accompanying properties of a strained single-crystal monolayer WS2of submicron scale were investigated using a theoretical-experimental joint study. After thermal strain, the WS2monolayer was split into different forms by several cracks, with the cause of the crack formation being studied using finite element analysis (FEA). The cracks were initiated from the vertex of the nucleation center, extending along the stronger von Mises stress isolines and terminating at the edges of the monolayers. Within the separate sections, ripple regions were observed, forming several typical nanopatterns. The band gap, frictional, viscosity, and elasticity characteristics of the different strain regions were also investigated. The nanopattern should enable flexibility in the design of more sophisticated devices based on 2D materials.
UR - http://www.scopus.com/inward/record.url?scp=85128669302&partnerID=8YFLogxK
U2 - 10.1021/acs.jpcc.1c10538
DO - 10.1021/acs.jpcc.1c10538
M3 - Article
AN - SCOPUS:85128669302
SN - 1932-7447
VL - 126
SP - 7184
EP - 7192
JO - Journal of Physical Chemistry C
JF - Journal of Physical Chemistry C
IS - 16
ER -