Two-dimensional electronic spectroscopy for mapping molecular photophysics

Jessica M. Anna, Yin Song, Rayomond Dinshaw, Gregory D. Scholes

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Abstract

We demonstrate the ability of two-dimensional electronic spectroscopy (2DES) to map ultrafast energy transfer and dynamics in two systems: the pigment-protein complex photosystem I (PSI) and aggregates of the conjugated polymer poly(3-hexylthiophene) (P3HT). A detailed description of our experimental set-up and data processing procedure is also given.

Original languageEnglish
Pages (from-to)1307-1319
Number of pages13
JournalPure and Applied Chemistry
Volume85
Issue number7
DOIs
Publication statusPublished - 2013
Externally publishedYes

Keywords

  • Energy transfer
  • Light harvesting
  • Molecular aggregates
  • Phasing
  • Photosynthesis
  • Two-dimensional electronic spectroscopy
  • Ultrafast spectroscopy

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Anna, J. M., Song, Y., Dinshaw, R., & Scholes, G. D. (2013). Two-dimensional electronic spectroscopy for mapping molecular photophysics. Pure and Applied Chemistry, 85(7), 1307-1319. https://doi.org/10.1351/PAC-CON-12-10-21