Study on Synthesis and Characterization of Bipyridine Ligated Scandium Complex ((C20H30N2)Sc(CH2SiMe3)3(THF)) and Its Catalytic Performance in Polymerization of Polar Conjugated Dienes

Qiaozhen Li, Mingqi Wang, Xiaofang Li*

*Corresponding author for this work

Research output: Chapter in Book/Report/Conference proceedingConference contributionpeer-review

Abstract

The highly cis-1,4 functionalized polyconjugated dienes was prepared by high-position/stereoregular coordination polymerization of poly(conjugated dienes)s can effectively introduce a number of heteroatom groups into synthetic rubbers, but it cannot only effectively improve the performance of synthetic rubber, but also develop new functional polyconjugated diene materials to broaden its application range. However, the rare earth metal catalysts that can promote the coordination polymerization of polar conjugated diene monomers are currently very limited. The bipyridine complex ((C20H30N2)Sc(CH2SiMe3)3(THF)) was simply synthesized using bipyridyl derivative ligand and equal amounts of Sc(CH2SiMe3)3(THF)2. For the bipyridyl-scandium trialkyl complex, different feeding ratios of cocatalyst borate can produce different catalytically active species. These generated catalytically active species can achieve coordination polymerization of polar 2-(2-methoxyphenyl)-1,3-butadiene.

Original languageEnglish
Title of host publicationFourth International Conference on Optoelectronic Science and Materials, ICOSM 2022
EditorsYuan Lu
PublisherSPIE
ISBN (Electronic)9781510662209
DOIs
Publication statusPublished - 2023
Event4th International Conference on Optoelectronic Science and Materials, ICOSM 2022 - Henfei, China
Duration: 16 Sept 202218 Sept 2022

Publication series

NameProceedings of SPIE - The International Society for Optical Engineering
Volume12553
ISSN (Print)0277-786X
ISSN (Electronic)1996-756X

Conference

Conference4th International Conference on Optoelectronic Science and Materials, ICOSM 2022
Country/TerritoryChina
CityHenfei
Period16/09/2218/09/22

Keywords

  • polar conjugated dienes
  • position/stereoselectivity
  • scandium catalyst

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