Photoinduced-electron-transfer-driven surface modification to regulate adsorption behavior in a pyridinium-decorated metal-organic framework

Xiao Dong Yang; Na Gao; Shuai Ma; Jing Wang Cui; Meng Ze Jia; Jie Zhang

doi:10.1039/c9cc06416h

Photoinduced-electron-transfer-driven surface modification to regulate adsorption behavior in a pyridinium-decorated metal-organic framework

Xiao Dong Yang, Na Gao, Shuai Ma, Jing Wang Cui, Meng Ze Jia, Jie Zhang^*

^*Corresponding author for this work

School of Chemistry and Chemical Engineering

Beijing Institute of Technology

Research output: Contribution to journal › Article › peer-review

19 Citations (Scopus)

Abstract

Surface modification based on a photo-induced electron transfer (PET) reaction in a pyridinium-decorated MOF material was found to be effective in regulating adsorption capacity. The current system enables the adsorption behavior to be manipulated based on variable affinity toward guest molecules through the redistribution of charge population with the preservation of the original pore structure, which is different from the prevalent approaches depending on photoinduced changes in molecular configurations of the pore backbone.

Original language	English
Pages (from-to)	12829-12832
Number of pages	4
Journal	Chemical Communications
Volume	55
Issue number	85
DOIs	https://doi.org/10.1039/c9cc06416h
Publication status	Published - 2019

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Yang, X. D., Gao, N., Ma, S., Cui, J. W., Jia, M. Z., & Zhang, J. (2019). Photoinduced-electron-transfer-driven surface modification to regulate adsorption behavior in a pyridinium-decorated metal-organic framework. Chemical Communications, 55(85), 12829-12832. https://doi.org/10.1039/c9cc06416h

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abstract = "Surface modification based on a photo-induced electron transfer (PET) reaction in a pyridinium-decorated MOF material was found to be effective in regulating adsorption capacity. The current system enables the adsorption behavior to be manipulated based on variable affinity toward guest molecules through the redistribution of charge population with the preservation of the original pore structure, which is different from the prevalent approaches depending on photoinduced changes in molecular configurations of the pore backbone.",

author = "Yang, {Xiao Dong} and Na Gao and Shuai Ma and Cui, {Jing Wang} and Jia, {Meng Ze} and Jie Zhang",

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AU - Gao, Na

AU - Ma, Shuai

AU - Cui, Jing Wang

AU - Jia, Meng Ze

AU - Zhang, Jie

PY - 2019

Y1 - 2019

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AB - Surface modification based on a photo-induced electron transfer (PET) reaction in a pyridinium-decorated MOF material was found to be effective in regulating adsorption capacity. The current system enables the adsorption behavior to be manipulated based on variable affinity toward guest molecules through the redistribution of charge population with the preservation of the original pore structure, which is different from the prevalent approaches depending on photoinduced changes in molecular configurations of the pore backbone.

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Photoinduced-electron-transfer-driven surface modification to regulate adsorption behavior in a pyridinium-decorated metal-organic framework

Abstract

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