Octave-spanning hyperspectral coherent diffractive imaging in the extreme ultraviolet range

Yijian Meng, Chunmei Zhang, Claude Marceau, A. Yu Naumov, P. B. Corkum, D. M. Villeneuve

Research output: Contribution to journalArticlepeer-review

18 Citations (Scopus)

Abstract

Soft x-ray microscopy is a powerful imaging technique that provides sub-micron spatial resolution, as well as chemical specificity using core-level near-edge x-ray absorption fine structure (NEXAFS). Near the carbon K-edge (280-300 eV) biological samples exhibit high contrast, and the detailed spectrum contains information about the local chemical environment of the atoms. Most soft x-ray imaging takes place on dedicated beamlines at synchrotron facilities or at x-ray free electron laser facilities. Tabletop femtosecond laser systems are now able to produce coherent radiation at the carbon K-edge and beyond through the process of high harmonic generation (HHG). The broad bandwidth of HHG is seemingly a limitation to imaging, since x-ray optical elements such as Fresnel zone plates require monochromatic sources. Counter-intuitively, the broad bandwidth of HHG sources can be beneficial as it permits chemicallyspecific hyperspectral imaging. We apply two separate techniques - Fourier transform spectroscopy, and lensless holographic imaging - To obtain images of an object simultaneously at multiple wavelengths using an octave-spanning high harmonic source with photon energies up to 30 eV. We use an interferometric delay reference to correct for nanometer-scale fluctuations between the two HHG sources.

Original languageEnglish
Pages (from-to)28960-28969
Number of pages10
JournalOptics Express
Volume23
Issue number22
DOIs
Publication statusPublished - 2 Nov 2015
Externally publishedYes

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