Low Dose Photoelectron Spectroscopy at BESSY II: Electronic structure of matter in its native state

Erika Giangrisostomi*, Ruslan Ovsyannikov, Florian Sorgenfrei, Teng Zhang, Andreas Lindblad, Yasmine Sassa, Ute B. Cappel, Torsten Leitner, Rolf Mitzner, Svante Svensson, Nils Mårtensson, Alexander Föhlisch

*Corresponding author for this work

Research output: Contribution to journalArticlepeer-review

36 Citations (Scopus)

Abstract

The implementation of a high-transmission, angular-resolved time-of-flight electron spectrometer with a 1.25 MHz pulse selector at the PM4 soft X-ray dipole beamline of the synchrotron BESSY II creates unique capabilities to inquire electronic structure via photoelectron spectroscopy with a minimum of radiation dose. Solid-state samples can be prepared and characterized with standard UHV techniques and rapidly transferred from various preparation chambers to a 4-axis temperature-controlled measurement stage. A synchronized MHz laser system enables excited-state characterization and dynamical studies starting from the picosecond timescale. This article introduces the principal characteristics of the PM4 beamline and LowDosePES end-station. Recent results from graphene, an organic hole transport material for solar cells and the transition metal dichalcogenide MoS2 are presented to demonstrate the instrument performances.

Original languageEnglish
Pages (from-to)68-78
Number of pages11
JournalJournal of Electron Spectroscopy and Related Phenomena
Volume224
DOIs
Publication statusPublished - Apr 2018
Externally publishedYes

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