Growth and Characterization of CrK(SO4)2•12H2O Crystals Used in Magnetic Adiabatic Refrigerator

Yuwei Chen, Ping Liu, Wang Liu, Chang Wang, Wei Dai, Jun Shen, Guochun Zhang, Heng Tu*

*Corresponding author for this work

Research output: Contribution to journalArticlepeer-review

Abstract

Paramagnetic salts perform satisfactorily in cryogenic refrigeration, and hydrated salt crystals are usually used as refrigerated materials at a rather low temperature. In this paper, a chromium potassium alum CrK(SO4)2•12H2O (CPA) single crystal with the size of 32 mm×32 mm×20 mm was grown by a slow cooling method. The relationship between the growth condition and crystal morphology was analyzed, and the thermal behavior, infrared spectrum, and magnetic performance of CPA crystal were also investigated. The results reveal that the CPA crystal exhibits a magnetocaloric effect up to 29.75 J•kg-1•K-1 in an applied magnetic field of 7 T at 2 K. A salt pill made by growing the CPA crystals on an array of copper wires in a sealed container was used in a two-stage single-shot adiabatic demagnetization refrigerator, obtaining a no-load temperature of 90 mK.

Translated title of the contributionCrK(SO4)2•12H2O晶体的生长及其磁制冷性能
Original languageEnglish
Pages (from-to)3270-3275
Number of pages6
JournalKuei Suan Jen Hsueh Pao/ Journal of the Chinese Ceramic Society
Volume50
Issue number12
DOIs
Publication statusPublished - Dec 2022
Externally publishedYes

Keywords

  • Crystal growth
  • Crystal morphology
  • Magnetocaloric effect
  • Paramagnetic materials

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