Core-shell nanostructured organic redox polymer cathodes with superior performance

He Jia, Ting Quan, Xuelian Liu, Lu Bai, Jiande Wang, Fadoi Boujioui, Ran Ye, Alexandru Vlad, Yan Lu, Jean François Gohy*

*Corresponding author for this work

Research output: Contribution to journalArticlepeer-review

28 Citations (Scopus)

Abstract

Core-shell nanoparticles stabilized by a cationic surfactant are prepared from the poly(2,2,6,6-tetramethylpiperidinyloxy-4-yl methacrylate) redox polymer. The nanoparticles are further self-assembled with negatively charged reduced graphene oxide nanosheets and negatively charged multi-walled carbon nanotubes. This results in the formation of a free-standing cathode with a layered nanostructure and a high content of redox polymer that exhibits 100% utilization of the active substance with a measured capacity as high as 105 mAh/g based on the whole weight of the electrode.

Original languageEnglish
Article number103949
JournalNano Energy
Volume64
DOIs
Publication statusPublished - Oct 2019
Externally publishedYes

Keywords

  • Energy storage
  • Lithium ion battery
  • Nanostructured
  • Organic electrode
  • Redox polymer

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