TY - JOUR
T1 - Coexisting Ferromagnetic-Antiferromagnetic Phases and Manipulation in a Magnetic Topological Insulator MnBi4Te7
AU - Guo, Jianfeng
AU - Wang, Huan
AU - Wang, Xueyun
AU - Gu, Shangzhi
AU - Mi, Shuo
AU - Zhu, Shiyu
AU - Hu, Jiawei
AU - Pang, Fei
AU - Ji, Wei
AU - Gao, Hong Jun
AU - Xia, Tianlong
AU - Cheng, Zhihai
N1 - Publisher Copyright:
© 2022 American Chemical Society. All rights reserved.
PY - 2022/8/18
Y1 - 2022/8/18
N2 - Magnetic topological insulators (MTIs) have received considerable attention owing to the demonstration of various quantum phenomena, such as the quantum anomalous Hall effect and topological magnetoelectric effect. The intrinsic superlattice-like layered MTIs MnBi2Te4/(Bi2Te3)nhave been extensively investigated mainly through transport measurements; however, a direct investigation of their superlattice-sensitive magnetic behaviors is relatively rare. In this paper, we report a microscopic real-space investigation of the magnetic phase behaviors in MnBi4Te7using cryogenic magnetic force microscopy. The intrinsic robust A-type antiferromagnetic (AFM), surface spin-flip (SSF) + AFM, ferromagnetic (FM) + SSF + AFM, and forced FM phases are sequentially visualized via the increased external magnetic field, consistent with the magnetic behavior in the M-H curve. The temperature-dependent magnetic phase evolution behaviors are further investigated to obtain a complete H-T phase diagram of MnBi4Te7. Tentative local phase manipulation via the stray field of the magnetic tip is demonstrated by transforming the AFM into the FM phase in the surface layers of MnBi4Te7. Our study provides key real-space ingredients for understanding the complicated magnetic, electronic, and topological properties of such intrinsic MTIs and suggests new directions for manipulating spin textures and locally controlling their exotic properties.
AB - Magnetic topological insulators (MTIs) have received considerable attention owing to the demonstration of various quantum phenomena, such as the quantum anomalous Hall effect and topological magnetoelectric effect. The intrinsic superlattice-like layered MTIs MnBi2Te4/(Bi2Te3)nhave been extensively investigated mainly through transport measurements; however, a direct investigation of their superlattice-sensitive magnetic behaviors is relatively rare. In this paper, we report a microscopic real-space investigation of the magnetic phase behaviors in MnBi4Te7using cryogenic magnetic force microscopy. The intrinsic robust A-type antiferromagnetic (AFM), surface spin-flip (SSF) + AFM, ferromagnetic (FM) + SSF + AFM, and forced FM phases are sequentially visualized via the increased external magnetic field, consistent with the magnetic behavior in the M-H curve. The temperature-dependent magnetic phase evolution behaviors are further investigated to obtain a complete H-T phase diagram of MnBi4Te7. Tentative local phase manipulation via the stray field of the magnetic tip is demonstrated by transforming the AFM into the FM phase in the surface layers of MnBi4Te7. Our study provides key real-space ingredients for understanding the complicated magnetic, electronic, and topological properties of such intrinsic MTIs and suggests new directions for manipulating spin textures and locally controlling their exotic properties.
UR - http://www.scopus.com/inward/record.url?scp=85136283490&partnerID=8YFLogxK
U2 - 10.1021/acs.jpcc.2c02223
DO - 10.1021/acs.jpcc.2c02223
M3 - Article
AN - SCOPUS:85136283490
SN - 1932-7447
VL - 126
SP - 13884
EP - 13893
JO - Journal of Physical Chemistry C
JF - Journal of Physical Chemistry C
IS - 32
ER -