TY - JOUR
T1 - An extended moments model of quantum efficiency for metals and semiconductors
AU - Jensen, Kevin L.
AU - Shabaev, Andrew
AU - Lambrakos, Samuel G.
AU - Finkenstadt, Daniel
AU - Petillo, John J.
AU - Alexander, Anna M.
AU - Smedley, John
AU - Moody, Nathan A.
AU - Yamaguchi, Hisato
AU - Liu, Fangze
AU - Neukirch, Amanda J.
AU - Tretiak, Sergei
N1 - Publisher Copyright:
© 2020 U.S. Government.
PY - 2020/7/7
Y1 - 2020/7/7
N2 - The complexity of photocathode designs and detector materials, and the need to model their performance for short pulse durations, the response to high-frequency photons, the presence of coatings and/or thinness of the absorptive layer, necessitates modifications to three-step and moments models of photoemission that are used in simulation codes. In this study, methods to include input from computationally intensive approaches, such as density functional theory to model optical properties and transfer matrix approaches to treat emission from the surface or transport past coatings, by means of parametric models are demonstrated. First, a technique to accurately represent optical behavior so as to model reflectivity and penetration depth is given. Second, modifications to bulk models arising from the usage of thin film architectures, and a means to rapidly calculate them, are provided. Third, a parameterization to model the impact of wells associated with coatings and surface layers on the transmission probably is given. In all cases, the methods are computationally efficient and designed to allow for including input from numerically intensive approaches that would otherwise be unavailable for simulations.
AB - The complexity of photocathode designs and detector materials, and the need to model their performance for short pulse durations, the response to high-frequency photons, the presence of coatings and/or thinness of the absorptive layer, necessitates modifications to three-step and moments models of photoemission that are used in simulation codes. In this study, methods to include input from computationally intensive approaches, such as density functional theory to model optical properties and transfer matrix approaches to treat emission from the surface or transport past coatings, by means of parametric models are demonstrated. First, a technique to accurately represent optical behavior so as to model reflectivity and penetration depth is given. Second, modifications to bulk models arising from the usage of thin film architectures, and a means to rapidly calculate them, are provided. Third, a parameterization to model the impact of wells associated with coatings and surface layers on the transmission probably is given. In all cases, the methods are computationally efficient and designed to allow for including input from numerically intensive approaches that would otherwise be unavailable for simulations.
UR - http://www.scopus.com/inward/record.url?scp=85087617369&partnerID=8YFLogxK
U2 - 10.1063/5.0011145
DO - 10.1063/5.0011145
M3 - Article
AN - SCOPUS:85087617369
SN - 0021-8979
VL - 128
JO - Journal of Applied Physics
JF - Journal of Applied Physics
IS - 1
M1 - 015301
ER -