A route toward digital manipulation of water nanodroplets on surfaces

Meng Cheng, Duoming Wang, Zhaoru Sun, Jing Zhao, Rong Yang, Guole Wang, Wei Yang, Guibai Xie, Jing Zhang, Peng Chen, Congli He, Donghua Liu, Limei Xu, Dongxia Shi, Enge Wang, Guangyu Zhang*

*Corresponding author for this work

Research output: Contribution to journalArticlepeer-review

36 Citations (Scopus)

Abstract

Manipulation of an isolated water nanodroplet (WN) on certain surfaces is important to various nanofluidic applications but challenging. Here we present a digital nanofluidic system based on a graphene/water/mica sandwich structure. In this architecture, graphene provides a flexible protection layer to isolate WNs from the outside environment, and a monolayer ice-like layer formed on the mica surface acts as a lubricant layer to allow these trapped WNs to move on it freely. In combination with scanning probe microscope techniques, we are able to move, merge, and separate individual water nanodroplets in a controlled manner. The smallest manipulatable water nanodroplet has a volume down to yoctoliter (10-24 L) scale.

Original languageEnglish
Pages (from-to)3955-3960
Number of pages6
JournalACS Nano
Volume8
Issue number4
DOIs
Publication statusPublished - 22 Apr 2014
Externally publishedYes

Keywords

  • atomic force microscope
  • graphene cover
  • ice-like layer
  • molecular dynamics simulation
  • nanofluidic manipulation

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