Activation of persulfates by carbonaceous materials: A review

Wuqi Huang, Sa Xiao, Hua Zhong*, Ming Yan, Xin Yang

*此作品的通讯作者

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369 引用 (Scopus)

摘要

In recent years, persulfate-based advanced oxidation processes (PS-AOPs) for removal of organic contaminants from water have gained wide attention. Ever-emerging carbonaceous materials, including pristine carbon materials and their derivatives, heteroatom-doped carbon materials, and carbon materials with metal particles, are demonstrated to be effective in the activation of persulfates (peroxymonosulfate (PMS) and peroxydisulfate (PDS)) to generate free radicals or non-radical active species for degradation of the contaminants. In this paper, mechanisms for the activation of persulfates by carbonaceous materials and their composites are analyzed and summarized. In particular, the synergistic effect for activation improvement in the composites or in the hybrid activation systems is explored. Then the influence of the environmental conditions, such as pH, temperature, inorganic anions and dissolved organic matter, on the activation processes are discussed. Deactivation and regeneration of the carbonaceous materials are discussed as well. Finally, the application of these carbonaceous materials in activating persulfates for remediation of contaminated groundwater and treatment of wastewater are reviewed and the challenges for such applications are proposed.

源语言英语
文章编号129297
期刊Chemical Engineering Journal
418
DOI
出版状态已出版 - 15 8月 2021
已对外发布

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Huang, W., Xiao, S., Zhong, H., Yan, M., & Yang, X. (2021). Activation of persulfates by carbonaceous materials: A review. Chemical Engineering Journal, 418, 文章 129297. https://doi.org/10.1016/j.cej.2021.129297