Solvothermal synthesis and characterization of a new titanium phosphate with a one-dimensional chiral chain

Y. Guo, Z. Shi, J. Yu, J. Wang, Y. Liu, N. Bai, W. Pang*

*Corresponding author for this work

Research output: Contribution to journalArticlepeer-review

43 Citations (Scopus)

Abstract

A new titanium phosphate, [Ti3P6O27]·5[NH3 CH2CH2NH3]·2[H3O], denoted JTP-A (Jilintitanium phosphate-A), has been synthesized under solvothermal conditions and its structure determined by single-crystal X-ray diffraction. It crystallizes in an enantiomorphic space group P212121 with lattice parameters a = 10.1800(6) Å, b = 15.8992(9) Å, c = 23.2271(12) Å, V = 3759(4) Å3, and Z = 4. The structure consists of one-dimensional chiral chains built up from corner-sharing titanium oxo octahedra running along the 21-screw axis, with the adjacent titanium oxo octahedra being bridged by phosphate tetrehedra. The Ti - O bond lengths along the backbone of the chain are alternately short and long. The results of TGA, IR, 31P MAS NMR, and second harmonics generation measurements are also presented.

Original languageEnglish
Pages (from-to)203-207
Number of pages5
JournalChemistry of Materials
Volume13
Issue number1
DOIs
Publication statusPublished - 2001
Externally publishedYes

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