An amino acid-assisted approach to fabricate nanosized hierarchical TS-1 zeolites for efficient oxidative desulfurization

Guoju Yang; Ji Han; Ziyi Qiu; Xiaoxin Chen; Zhaochi Feng; Jihong Yu

doi:10.1039/c9qi01543d

An amino acid-assisted approach to fabricate nanosized hierarchical TS-1 zeolites for efficient oxidative desulfurization

Guoju Yang, Ji Han, Ziyi Qiu, Xiaoxin Chen^*, Zhaochi Feng, Jihong Yu

^*Corresponding author for this work

Research output: Contribution to journal › Article › peer-review

48 Citations (Scopus)

Abstract

Nanosized hierarchical TS-1 zeolites with intercrystalline and intracrystalline meso-/macropores have been successfully synthesised by amino acid-assisted strategy under two-step rota-crystallization conditions. Compared to micron-sized microporous TS-1 zeolites, amino acid-directed hierarchical materials exhibit remarkably enhanced catalytic activity in oxidative desulfurization reactions owing to the improved accessibility of reactants to the microporous space of zeolites.

Original language	English
Pages (from-to)	1975-1980
Number of pages	6
Journal	Inorganic Chemistry Frontiers
Volume	7
Issue number	10
DOIs	https://doi.org/10.1039/c9qi01543d
Publication status	Published - 21 May 2020
Externally published	Yes

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abstract = "Nanosized hierarchical TS-1 zeolites with intercrystalline and intracrystalline meso-/macropores have been successfully synthesised by amino acid-assisted strategy under two-step rota-crystallization conditions. Compared to micron-sized microporous TS-1 zeolites, amino acid-directed hierarchical materials exhibit remarkably enhanced catalytic activity in oxidative desulfurization reactions owing to the improved accessibility of reactants to the microporous space of zeolites.",

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AU - Yang, Guoju

AU - Han, Ji

AU - Qiu, Ziyi

AU - Chen, Xiaoxin

AU - Feng, Zhaochi

AU - Yu, Jihong

PY - 2020/5/21

Y1 - 2020/5/21

N2 - Nanosized hierarchical TS-1 zeolites with intercrystalline and intracrystalline meso-/macropores have been successfully synthesised by amino acid-assisted strategy under two-step rota-crystallization conditions. Compared to micron-sized microporous TS-1 zeolites, amino acid-directed hierarchical materials exhibit remarkably enhanced catalytic activity in oxidative desulfurization reactions owing to the improved accessibility of reactants to the microporous space of zeolites.

AB - Nanosized hierarchical TS-1 zeolites with intercrystalline and intracrystalline meso-/macropores have been successfully synthesised by amino acid-assisted strategy under two-step rota-crystallization conditions. Compared to micron-sized microporous TS-1 zeolites, amino acid-directed hierarchical materials exhibit remarkably enhanced catalytic activity in oxidative desulfurization reactions owing to the improved accessibility of reactants to the microporous space of zeolites.

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DO - 10.1039/c9qi01543d

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An amino acid-assisted approach to fabricate nanosized hierarchical TS-1 zeolites for efficient oxidative desulfurization

Abstract

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