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Pressure-induced superconductivity extending across the topological phase transition in thallium-based topological materials

  • Cuiying Pei
  • , Peihao Huang
  • , Peng Zhu
  • , Linlin Liu
  • , Qi Wang
  • , Yi Zhao
  • , Lingling Gao
  • , Changhua Li
  • , Weizheng Cao
  • , Jian Lv
  • , Xiang Li
  • , Zhiwei Wang*
  • , Yugui Yao
  • , Binghai Yan*
  • , Claudia Felser
  • , Yulin Chen
  • , Hanyu Liu*
  • , Yanpeng Qi*
  • *此作品的通讯作者
  • ShanghaiTech University
  • Jilin University
  • Beijing Institute of Technology
  • Weizmann Institute of Science
  • Max Planck Institute for Chemical Physics of Solids
  • University of Oxford

科研成果: 期刊稿件文章同行评审

摘要

The coexistence of superconductivity and topology holds the potential to realize exotic quantum states of matter. Here, we report superconductivity induced by high pressure in three thallium-based materials, covering the phase transition from a normal insulator (TlBiS2) to a topological insulator (TlBiSe2) through a Dirac semimetal (TlBiSeS). By increasing the pressure up to 60 GPa, we observe superconductivity phase diagrams with maximal critical temperature (Tc) values at 6.0–8.1 K. Our density functional theory calculations reveal topological surface states in superconductivity phases for all three compounds. Our study paves the path to explore topological superconductivity and topological phase transitions.

源语言英语
文章编号101094
期刊Cell Reports Physical Science
3
10
DOI
出版状态已出版 - 19 10月 2022

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