TY - JOUR
T1 - Polarization Signal Amplification of 2D GeSe-Based Polarization-Sensitive Photodetectors
AU - He, Kexin
AU - Ran, Wenhao
AU - Xu, Shaodi
AU - Wen, Jie
AU - Qiu, Siqi
AU - Liu, Tingwei
AU - Xin, Kaiyao
AU - Yu, Yali
AU - Liu, Duan Yang
AU - Huang, Qianqian
AU - Shen, Guozhen
AU - Wei, Zhongming
AU - Zhou, Ziqi
N1 - Publisher Copyright:
© 2025 Wiley-VCH GmbH.
PY - 2025/10/2
Y1 - 2025/10/2
N2 - Polarization-sensitive photodetectors, resolving light intensity, wavelength, and polarization states, enable the characterization of probing microstructure, internal stress, and compositional heterogeneity. Polarizer-free polarization-sensitive photodetectors based on in-plane anisotropic 2D semiconductors offer potential for device miniaturization and on-chip integration, owing to their inherent linear dichroism and orientation-dependent carrier mobilities. Hundreds of in-plane anisotropic 2D materials have been successfully discovered; however, the limited anisotropic photocurrent ratio (PR<10) has hindered the practical application. Herein, a field-effect transistor (FET)-based amplification strategy, enhancing PR from 2.1 to 54.8 in 2D GeSe photodetectors is proposed. This significant PR enhancement arises from polarization-induced resistance variations dynamically modulating gate potentials. Coupled with a steep transistor subthreshold region, small gate fluctuations produce substantial drain current changes, amplifying output anisotropy sensitively. Evaluating four types of FET identifies SMT-Si transistors as optimal due to their high stability, sharp subthreshold, and excellent noise immunity. In addition, the amplified PR signal directly enhances image contrast and recognition accuracy. Notably, with a high-PR signal, the machine learning model achieves a recognition rate of 0.99 in only 17 training epochs, reflecting a computational cost reduction of over 60%. This work provides an effective strategy to enhance PR, benefiting from high-resolution polarization imaging and advanced optoelectronic sensing.
AB - Polarization-sensitive photodetectors, resolving light intensity, wavelength, and polarization states, enable the characterization of probing microstructure, internal stress, and compositional heterogeneity. Polarizer-free polarization-sensitive photodetectors based on in-plane anisotropic 2D semiconductors offer potential for device miniaturization and on-chip integration, owing to their inherent linear dichroism and orientation-dependent carrier mobilities. Hundreds of in-plane anisotropic 2D materials have been successfully discovered; however, the limited anisotropic photocurrent ratio (PR<10) has hindered the practical application. Herein, a field-effect transistor (FET)-based amplification strategy, enhancing PR from 2.1 to 54.8 in 2D GeSe photodetectors is proposed. This significant PR enhancement arises from polarization-induced resistance variations dynamically modulating gate potentials. Coupled with a steep transistor subthreshold region, small gate fluctuations produce substantial drain current changes, amplifying output anisotropy sensitively. Evaluating four types of FET identifies SMT-Si transistors as optimal due to their high stability, sharp subthreshold, and excellent noise immunity. In addition, the amplified PR signal directly enhances image contrast and recognition accuracy. Notably, with a high-PR signal, the machine learning model achieves a recognition rate of 0.99 in only 17 training epochs, reflecting a computational cost reduction of over 60%. This work provides an effective strategy to enhance PR, benefiting from high-resolution polarization imaging and advanced optoelectronic sensing.
KW - 2D
KW - GeSe
KW - field-effect transistor
KW - polarization ratio
KW - polarization-sensitive photodetectors
UR - https://www.scopus.com/pages/publications/105009791978
U2 - 10.1002/adma.202509066
DO - 10.1002/adma.202509066
M3 - Article
C2 - 40613247
AN - SCOPUS:105009791978
SN - 0935-9648
VL - 37
JO - Advanced Materials
JF - Advanced Materials
IS - 39
M1 - 2509066
ER -