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Dominant Two-Dimensional Electron-Phonon Interactions in the Bulk Dirac Semimetal Na3Bi

  • Dhruv C. Desai
  • , Jinsoo Park
  • , Jin Jian Zhou
  • , Marco Bernardi*
  • *此作品的通讯作者
  • California Institute of Technology

科研成果: 期刊稿件文章同行评审

摘要

Bulk Dirac semimetals (DSMs) exhibit unconventional transport properties and phase transitions due to their peculiar low-energy band structure, yet the electronic interactions governing nonequilibrium phenomena in DSMs are not fully understood. Here we show that electron-phonon (e-ph) interactions in a prototypical bulk DSM, Na3Bi, are predominantly two-dimensional (2D). Our first-principles calculations reveal a 2D optical phonon with strong e-ph interactions associated with in-plane vibrations of Na atoms. We show that this 2D mode governs e-ph scattering and charge transport in Na3Bi and induces a dynamical phase transition to a Weyl semimetal. Our work advances the quantitative analysis of electron interactions in Na3Bi and reveals a dominant low-dimensional interaction in a bulk Dirac semimetal.

源语言英语
页(从-至)3947-3953
页数7
期刊Nano Letters
23
9
DOI
出版状态已出版 - 10 5月 2023

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