Solution-Processed Micro-Nanostructured Electron Transport Layer via Bubble-Assisted Assembly for Efficient Perovskite Photovoltaics

Yongrui Yang; Fanyi Min; Yiyang Wang; Lutong Guo; Haoran Long; Zhiyuan Qu; Kun Zhang; Yang Wang; Juehan Yang; Yu Chen; Lei Meng; Yali Qiao; Yanlin Song

doi:10.1002/adma.202408448

Solution-Processed Micro-Nanostructured Electron Transport Layer via Bubble-Assisted Assembly for Efficient Perovskite Photovoltaics

Yongrui Yang, Fanyi Min, Yiyang Wang, Lutong Guo, Haoran Long, Zhiyuan Qu, Kun Zhang, Yang Wang, Juehan Yang, Yu Chen, Lei Meng^*, Yali Qiao^*, Yanlin Song^*

^*Corresponding author for this work

Research output: Contribution to journal › Article › peer-review

10 Citations (Scopus)

Abstract

Organic–inorganic halide perovskite solar cells (PSCs) have attracted significant attention in photovoltaic research, owing to their superior optoelectronic properties and cost-effective manufacturing techniques. However, the unbalanced charge carrier diffusion length in perovskite materials leads to the recombination of photogenerated electrons and holes. The inefficient charge carrier collecting process severely affects the power conversion efficiency (PCE) of the PSCs. Herein, a solution-processed SnO₂ array electron transport layer with precisely tunable micro-nanostructures is fabricated via a bubble-template-assisted approach, serving as both electron transport layers and scaffolds for the perovskite layer. Due to the optimized electron transporting pathway and enlarged perovskite grain size, the PSCs achieve a PCE of 25.35% (25.07% certificated PCE).

Original language	English
Article number	2408448
Journal	Advanced Materials
Volume	36
Issue number	46
DOIs	https://doi.org/10.1002/adma.202408448
Publication status	Published - 14 Nov 2024
Externally published	Yes

Keywords

bubble-assisted patterning
charge carrier dynamics
micro-nanostructured interface
perovskite photovoltaics
solar cells

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

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10.1002/adma.202408448

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title = "Solution-Processed Micro-Nanostructured Electron Transport Layer via Bubble-Assisted Assembly for Efficient Perovskite Photovoltaics",

abstract = "Organic–inorganic halide perovskite solar cells (PSCs) have attracted significant attention in photovoltaic research, owing to their superior optoelectronic properties and cost-effective manufacturing techniques. However, the unbalanced charge carrier diffusion length in perovskite materials leads to the recombination of photogenerated electrons and holes. The inefficient charge carrier collecting process severely affects the power conversion efficiency (PCE) of the PSCs. Herein, a solution-processed SnO2 array electron transport layer with precisely tunable micro-nanostructures is fabricated via a bubble-template-assisted approach, serving as both electron transport layers and scaffolds for the perovskite layer. Due to the optimized electron transporting pathway and enlarged perovskite grain size, the PSCs achieve a PCE of 25.35\% (25.07\% certificated PCE).",

keywords = "bubble-assisted patterning, charge carrier dynamics, micro-nanostructured interface, perovskite photovoltaics, solar cells",

author = "Yongrui Yang and Fanyi Min and Yiyang Wang and Lutong Guo and Haoran Long and Zhiyuan Qu and Kun Zhang and Yang Wang and Juehan Yang and Yu Chen and Lei Meng and Yali Qiao and Yanlin Song",

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year = "2024",

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doi = "10.1002/adma.202408448",

language = "English",

volume = "36",

journal = "Advanced Materials",

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T1 - Solution-Processed Micro-Nanostructured Electron Transport Layer via Bubble-Assisted Assembly for Efficient Perovskite Photovoltaics

AU - Yang, Yongrui

AU - Min, Fanyi

AU - Wang, Yiyang

AU - Guo, Lutong

AU - Long, Haoran

AU - Qu, Zhiyuan

AU - Zhang, Kun

AU - Wang, Yang

AU - Yang, Juehan

AU - Chen, Yu

AU - Meng, Lei

AU - Qiao, Yali

AU - Song, Yanlin

PY - 2024/11/14

Y1 - 2024/11/14

N2 - Organic–inorganic halide perovskite solar cells (PSCs) have attracted significant attention in photovoltaic research, owing to their superior optoelectronic properties and cost-effective manufacturing techniques. However, the unbalanced charge carrier diffusion length in perovskite materials leads to the recombination of photogenerated electrons and holes. The inefficient charge carrier collecting process severely affects the power conversion efficiency (PCE) of the PSCs. Herein, a solution-processed SnO2 array electron transport layer with precisely tunable micro-nanostructures is fabricated via a bubble-template-assisted approach, serving as both electron transport layers and scaffolds for the perovskite layer. Due to the optimized electron transporting pathway and enlarged perovskite grain size, the PSCs achieve a PCE of 25.35% (25.07% certificated PCE).

AB - Organic–inorganic halide perovskite solar cells (PSCs) have attracted significant attention in photovoltaic research, owing to their superior optoelectronic properties and cost-effective manufacturing techniques. However, the unbalanced charge carrier diffusion length in perovskite materials leads to the recombination of photogenerated electrons and holes. The inefficient charge carrier collecting process severely affects the power conversion efficiency (PCE) of the PSCs. Herein, a solution-processed SnO2 array electron transport layer with precisely tunable micro-nanostructures is fabricated via a bubble-template-assisted approach, serving as both electron transport layers and scaffolds for the perovskite layer. Due to the optimized electron transporting pathway and enlarged perovskite grain size, the PSCs achieve a PCE of 25.35% (25.07% certificated PCE).

KW - bubble-assisted patterning

KW - charge carrier dynamics

KW - micro-nanostructured interface

KW - perovskite photovoltaics

KW - solar cells

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U2 - 10.1002/adma.202408448

DO - 10.1002/adma.202408448

M3 - Article

C2 - 39328020

AN - SCOPUS:85204880023

SN - 0935-9648

VL - 36

JO - Advanced Materials

JF - Advanced Materials

IS - 46

M1 - 2408448

ER -

Solution-Processed Micro-Nanostructured Electron Transport Layer via Bubble-Assisted Assembly for Efficient Perovskite Photovoltaics

Abstract

Keywords

UN SDGs

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