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Revealing exciton transport in atomically thin semiconductors

  • Fengjiang Liu
  • , Kai Chen
  • , Wei Yan
  • , Weiwei Tang
  • , Hao Zhang
  • , Richard J. Blaikie
  • , Yu Hui Chen
  • , Boyang Ding
  • , Min Qiu
  • Westlake University
  • Dodd-Walls Centre for Photonic and Quantum Technologies
  • MacDiarmid Institute for Advanced Materials and Nanotechnology
  • Victoria University of Wellington
  • University of Otago
  • Coherent Scientific Pty. Ltd.

Research output: Contribution to journalArticlepeer-review

Abstract

Exciton transport is a fundamental process that underlies the functionality of semiconductor optoelectronic devices. However, when excitons interact with one another, their transport pattern becomes unpredictable, posing a great challenge to harness their full potential in various applications. In our study, focusing on the exciton density change in a tungsten-disulfide monolayer, we observed that strong interactions between excitons can actually stop their movement. This finding contradicts the typical understanding of consistent exciton movement and reveals that a higher density might decrease the exciton-exciton annihilation rate due to reduced mobility. Our findings offer a valuable technique to examine exciton transport and deepen our grasp of their behavior in many-body interactions, which could pave the way for better-performing excitonic devices.

Original languageEnglish
Article number205418
JournalPhysical Review B
Volume109
Issue number20
DOIs
Publication statusPublished - 15 May 2024

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