Enantiospecific state transfer for gaseous symmetric-top chiral molecules

We study the enantiospecific state transfer for gaseous symmetric-top chiral molecules by constructing a four-level model. This model is formed by coupling the electric dipole transitions among four appropriate rovibrational states with three electromagnetic fields. It includes two cyclic three-level substructures, where the overall phases of the coupling strengths differ by π with enantiomers and reflect the chirality dependence of the molecules. Based on this four-level model, two dynamic ways are proposed to achieve the approximately perfect enantiospecific state transfer for gaseous symmetric-top chiral molecules when all the molecules are initially in the ground state of the system.