Edge-Mediated Magnetic Domain Rearrangement in van der Waals Magnet Fe3GaTe2

Shuaizhao Jin, Yujia Liu, Baijun Gu, Xiangping Zhang, Yiting Wang, Yichong Chen, Tianlong Xia, Boyuan Huang, Jiawang Hong, Xueyun Wang*

*Corresponding author for this work

Research output: Contribution to journalArticlepeer-review

Abstract

The emergence of van der Waals (vdW) magnets has opened new frontiers for investigation of 2-dimensional magnetism and application of spintronic memories. However, as the system approached the nanoscale, the edge effect significantly enhanced, posing critical challenges in understanding edge-mediated modifications of magnetic behavior, such as the nanoscale magnetic domain. Here, we employ magnetic force microscopy to systematically investigate edge-mediated magnetic domain rearrangement in Fe3GaTe2 flakes. By performing thermal treatment, we observed a distinct transition from labyrinthine to edge-localized stripe domains perpendicular to the flake edges. Furthermore, we reveal a competition and stabilization between size effect and edge effect by investigating thickness-dependent variation in the length of stripe domains and indicate that such an edge effect suppresses the formation of skyrmions. These findings not only elucidate the critical role of the edge effect in governing the domain morphology of vdW magnets but also provide insights for designing edge-mediated nanostructures in next-generation spintronic devices.

Original languageEnglish
Pages (from-to)7885-7891
Number of pages7
JournalNano Letters
Volume25
Issue number19
DOIs
Publication statusPublished - 14 May 2025
Externally publishedYes

Keywords

  • Edge effect
  • FeGaTe
  • Magnetic domain
  • van der Waals magnet

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