Data–Knowledge-Dual-Driven Electrolyte Design for Fast-Charging Lithium Ion Batteries

Yi Yang; Nan Yao; Yu Chen Gao; Xiang Chen; Yu Xin Huang; Shuo Zhang; Han Bing Zhu; Lei Xu; Yu Xing Yao; Shi Jie Yang; Zheng Liao; Zeheng Li; Xue Fei Wen; Peng Wu; Ting Lu Song; Jin Hao Yao; Jiang Kui Hu; Chong Yan; Jia Qi Huang; Qiang Zhang

doi:10.1002/anie.202505212

Data–Knowledge-Dual-Driven Electrolyte Design for Fast-Charging Lithium Ion Batteries

Yi Yang, Nan Yao, Yu Chen Gao, Xiang Chen^*, Yu Xin Huang, Shuo Zhang, Han Bing Zhu, Lei Xu, Yu Xing Yao, Shi Jie Yang, Zheng Liao, Zeheng Li, Xue Fei Wen, Peng Wu, Ting Lu Song, Jin Hao Yao, Jiang Kui Hu, Chong Yan, Jia Qi Huang^*, Qiang Zhang^*

^*Corresponding author for this work

Advanced Research Institute of Multidisciplinary Science

Research output: Contribution to journal › Article › peer-review

Abstract

Electric vehicles (EVs) starve for minutes-level fast-charging lithium-ion batteries (LIBs), while the heat gathering at high-rate charging and torridity conditions has detrimental effects on electrolytes, triggering rapid battery degradation and even safety hazards. However, the current research on high-temperature fast-charging (HTFC) electrolytes is very lacking. We revolutionized the conventional paradigm of developing HTFC electrolytes integrating with high-throughput calculation, machine-learning techniques, and experimental verifications to establish a data–knowledge-dual-driven approach. Ethyl trimethylacetate was efficiently screened out based on the approach and enabled batteries to work under high temperatures with distinctly restricted side reactions. A stable and highly safe fast-charging (15-min charging to 80% capacity) cycling without Li plating was achieved over 4100 cycles at 45 °C based on 181 Wh kg⁻¹ pouch cells, demonstrating the state-of-the-art in this field.

Original language	English
Article number	e202505212
Journal	Angewandte Chemie - International Edition
Volume	64
Issue number	24
DOIs	https://doi.org/10.1002/anie.202505212
Publication status	Published - 10 Jun 2025

Keywords

Data–knowledge-dual-driven screening
Fast charging
High temperature
Lithium-ion batteries
Molecular design

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

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10.1002/anie.202505212

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Yang, Y., Yao, N., Gao, Y. C., Chen, X., Huang, Y. X., Zhang, S., Zhu, H. B., Xu, L., Yao, Y. X., Yang, S. J., Liao, Z., Li, Z., Wen, X. F., Wu, P., Song, T. L., Yao, J. H., Hu, J. K., Yan, C., Huang, J. Q., & Zhang, Q. (2025). Data–Knowledge-Dual-Driven Electrolyte Design for Fast-Charging Lithium Ion Batteries. Angewandte Chemie - International Edition, 64(24), Article e202505212. https://doi.org/10.1002/anie.202505212

@article{4afe78681a744766b7feca66ea375f7b,

title = "Data–Knowledge-Dual-Driven Electrolyte Design for Fast-Charging Lithium Ion Batteries",

abstract = "Electric vehicles (EVs) starve for minutes-level fast-charging lithium-ion batteries (LIBs), while the heat gathering at high-rate charging and torridity conditions has detrimental effects on electrolytes, triggering rapid battery degradation and even safety hazards. However, the current research on high-temperature fast-charging (HTFC) electrolytes is very lacking. We revolutionized the conventional paradigm of developing HTFC electrolytes integrating with high-throughput calculation, machine-learning techniques, and experimental verifications to establish a data–knowledge-dual-driven approach. Ethyl trimethylacetate was efficiently screened out based on the approach and enabled batteries to work under high temperatures with distinctly restricted side reactions. A stable and highly safe fast-charging (15-min charging to 80% capacity) cycling without Li plating was achieved over 4100 cycles at 45 °C based on 181 Wh kg−1 pouch cells, demonstrating the state-of-the-art in this field.",

keywords = "Data–knowledge-dual-driven screening, Fast charging, High temperature, Lithium-ion batteries, Molecular design",

author = "Yi Yang and Nan Yao and Gao, {Yu Chen} and Xiang Chen and Huang, {Yu Xin} and Shuo Zhang and Zhu, {Han Bing} and Lei Xu and Yao, {Yu Xing} and Yang, {Shi Jie} and Zheng Liao and Zeheng Li and Wen, {Xue Fei} and Peng Wu and Song, {Ting Lu} and Yao, {Jin Hao} and Hu, {Jiang Kui} and Chong Yan and Huang, {Jia Qi} and Qiang Zhang",

note = "Publisher Copyright: {\textcopyright} 2025 Wiley-VCH GmbH.",

year = "2025",

month = jun,

day = "10",

doi = "10.1002/anie.202505212",

language = "English",

volume = "64",

journal = "Angewandte Chemie - International Edition",

issn = "1433-7851",

publisher = "John Wiley and Sons Ltd",

number = "24",

}

Yang, Y, Yao, N, Gao, YC, Chen, X, Huang, YX, Zhang, S, Zhu, HB, Xu, L, Yao, YX, Yang, SJ, Liao, Z, Li, Z, Wen, XF, Wu, P, Song, TL, Yao, JH, Hu, JK, Yan, C , Huang, JQ & Zhang, Q 2025, 'Data–Knowledge-Dual-Driven Electrolyte Design for Fast-Charging Lithium Ion Batteries', Angewandte Chemie - International Edition, vol. 64, no. 24, e202505212. https://doi.org/10.1002/anie.202505212

TY - JOUR

T1 - Data–Knowledge-Dual-Driven Electrolyte Design for Fast-Charging Lithium Ion Batteries

AU - Yang, Yi

AU - Yao, Nan

AU - Gao, Yu Chen

AU - Chen, Xiang

AU - Huang, Yu Xin

AU - Zhang, Shuo

AU - Zhu, Han Bing

AU - Xu, Lei

AU - Yao, Yu Xing

AU - Yang, Shi Jie

AU - Liao, Zheng

AU - Li, Zeheng

AU - Wen, Xue Fei

AU - Wu, Peng

AU - Song, Ting Lu

AU - Yao, Jin Hao

AU - Hu, Jiang Kui

AU - Yan, Chong

AU - Huang, Jia Qi

AU - Zhang, Qiang

PY - 2025/6/10

Y1 - 2025/6/10

N2 - Electric vehicles (EVs) starve for minutes-level fast-charging lithium-ion batteries (LIBs), while the heat gathering at high-rate charging and torridity conditions has detrimental effects on electrolytes, triggering rapid battery degradation and even safety hazards. However, the current research on high-temperature fast-charging (HTFC) electrolytes is very lacking. We revolutionized the conventional paradigm of developing HTFC electrolytes integrating with high-throughput calculation, machine-learning techniques, and experimental verifications to establish a data–knowledge-dual-driven approach. Ethyl trimethylacetate was efficiently screened out based on the approach and enabled batteries to work under high temperatures with distinctly restricted side reactions. A stable and highly safe fast-charging (15-min charging to 80% capacity) cycling without Li plating was achieved over 4100 cycles at 45 °C based on 181 Wh kg−1 pouch cells, demonstrating the state-of-the-art in this field.

AB - Electric vehicles (EVs) starve for minutes-level fast-charging lithium-ion batteries (LIBs), while the heat gathering at high-rate charging and torridity conditions has detrimental effects on electrolytes, triggering rapid battery degradation and even safety hazards. However, the current research on high-temperature fast-charging (HTFC) electrolytes is very lacking. We revolutionized the conventional paradigm of developing HTFC electrolytes integrating with high-throughput calculation, machine-learning techniques, and experimental verifications to establish a data–knowledge-dual-driven approach. Ethyl trimethylacetate was efficiently screened out based on the approach and enabled batteries to work under high temperatures with distinctly restricted side reactions. A stable and highly safe fast-charging (15-min charging to 80% capacity) cycling without Li plating was achieved over 4100 cycles at 45 °C based on 181 Wh kg−1 pouch cells, demonstrating the state-of-the-art in this field.

KW - Data–knowledge-dual-driven screening

KW - Fast charging

KW - High temperature

KW - Lithium-ion batteries

KW - Molecular design

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U2 - 10.1002/anie.202505212

DO - 10.1002/anie.202505212

M3 - Article

AN - SCOPUS:105005077957

SN - 1433-7851

VL - 64

JO - Angewandte Chemie - International Edition

JF - Angewandte Chemie - International Edition

IS - 24

M1 - e202505212

ER -

Data–Knowledge-Dual-Driven Electrolyte Design for Fast-Charging Lithium Ion Batteries

Abstract

Keywords

UN SDGs

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