Attosecond light science and its application for probing quantum materials

  • Xun Shi*
  • , Chen Ting Liao
  • , Zhensheng Tao
  • , Emma Cating-Subramanian
  • , Margaret M. Murnane*
  • , Carlos Hernández-García
  • , Henry C. Kapteyn
  • *Corresponding author for this work

Research output: Contribution to journalArticlepeer-review

33 Citations (Scopus)

Abstract

In this paper, we review the development and application of coherent short wavelength light sources implemented using the high harmonic generation (HHG) process. The physics underlying HHG brought quantum physics into the domain of attosecond time-scales for the first time. The observation and manipulation of electron dynamics on such short time-scales - a capability not conceived - of just a few decades ago - is becoming both more-and-more sophisticated and useful as a route to achieve exquisite control over short wavelength light. New experimental techniques are enabling HHG light sources to provide new insights into fundamental quantum interactions in materials, making it possible for the first time to capture the fastest charge, spin, photon and phonon interactions and to achieve diffraction-limited imaging at short wavelengths.

Original languageEnglish
Article number184008
JournalJournal of Physics B: Atomic, Molecular and Optical Physics
Volume53
Issue number18
DOIs
Publication statusPublished - 28 Sept 2020
Externally publishedYes

Keywords

  • angle-resolved photoemission spectroscopy
  • attosecond
  • coherent diffraction imaging
  • high harmonic generation
  • spin and orbital angular momentum
  • ultrafast dynamics

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