TY - JOUR
T1 - A novel photoacoustic gas sensor for dual-component identification and concentration analysis
AU - Sun, Jiachen
AU - Wang, Fupeng
AU - Zhang, Lin
AU - Shao, Jiankun
N1 - Publisher Copyright:
© 2025
PY - 2025/3
Y1 - 2025/3
N2 - In this study, a neural network-assisted photoacoustic gas sensor is proposed that enables dual-component identification and concentration analysis of methane and ethylene, effectively addressing the issue of cross-interference in photoacoustic spectroscopy (PAS) technology. This sensor identifies the unknown photoacoustic second harmonic signal using a self-built photoacoustic deep neural network-component identification model, and then determines the composition of the gas sample. The traditional concentration fitting equation method and the self-built Photoacoustic Deep Neural Network-Concentration Regression Model are integrated to analyze the gas samples composed of single- and dual-component. The sensor demonstrates exceptionally high linearity, accuracy and robustness. Additionally, the minimum detection limits (MDLs) for a single-component are determined to be 0.28 ppm for methane and 1.56 ppm for ethylene. For dual-component detection, the MDLs are 8.86 ppm for methane and 4.55 ppm for ethylene. The promising results of the present study demonstrate that deep learning algorithm provides a more effective, accurate, and stable solution for elimination of cross-interference in photoacoustic gas sensor.
AB - In this study, a neural network-assisted photoacoustic gas sensor is proposed that enables dual-component identification and concentration analysis of methane and ethylene, effectively addressing the issue of cross-interference in photoacoustic spectroscopy (PAS) technology. This sensor identifies the unknown photoacoustic second harmonic signal using a self-built photoacoustic deep neural network-component identification model, and then determines the composition of the gas sample. The traditional concentration fitting equation method and the self-built Photoacoustic Deep Neural Network-Concentration Regression Model are integrated to analyze the gas samples composed of single- and dual-component. The sensor demonstrates exceptionally high linearity, accuracy and robustness. Additionally, the minimum detection limits (MDLs) for a single-component are determined to be 0.28 ppm for methane and 1.56 ppm for ethylene. For dual-component detection, the MDLs are 8.86 ppm for methane and 4.55 ppm for ethylene. The promising results of the present study demonstrate that deep learning algorithm provides a more effective, accurate, and stable solution for elimination of cross-interference in photoacoustic gas sensor.
KW - Cross-interference
KW - Dual-component identification
KW - Neural network
KW - Photoacoustic spectroscopy
UR - http://www.scopus.com/inward/record.url?scp=85213828129&partnerID=8YFLogxK
U2 - 10.1016/j.infrared.2025.105711
DO - 10.1016/j.infrared.2025.105711
M3 - Article
AN - SCOPUS:85213828129
SN - 1350-4495
VL - 145
JO - Infrared Physics and Technology
JF - Infrared Physics and Technology
M1 - 105711
ER -